Issue 6, 2015
From the journal:

New Journal of Chemistry

Heterogeneous Fe-MIL-101 catalysts for efficient one-pot four-component coupling synthesis of highly substituted pyrroles†

Jia Tang,a   Mu Yang,a   Ming Yang,a   Jingjing Wang,a   Wenjun Dong*a  and  Ge Wanga  

* Corresponding authors

a School of Materials Science and Engineering, University of Science and Technology Beijing, Beijing 100083, P. R. China
E-mail: wdong@ustb.edu.cn
Tel: +86-010-62333827

Abstract

Four-component coupling reactions (4CRs) of 1,3-dicarbonyl compounds, amines, aldehydes and nitromethane have been carried out for substituted pyrroles using iron-containing metal organic frameworks (MOFs) as heterogeneous catalysts. Due to its higher surface area and larger pore size, the Fe-MIL-101 catalyst exhibits higher activity than that of Fe-MIL-88B and Fe-MIL-53. The reusability and heterogeneity of the Fe-MIL-101 catalyst was investigated, and no significant reduction of its catalytic activity was observed over five cycles reaction.

Graphical abstract: Heterogeneous Fe-MIL-101 catalysts for efficient one-pot four-component coupling synthesis of highly substituted pyrroles

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Article information

DOI
https://doi.org/10.1039/C5NJ00632E
Article type
Paper
Submitted
13 Mar 2015
Accepted
16 Apr 2015
First published
23 Apr 2015

New J. Chem., 2015,39, 4919-4923

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Heterogeneous Fe-MIL-101 catalysts for efficient one-pot four-component coupling synthesis of highly substituted pyrroles

J. Tang, M. Yang, M. Yang, J. Wang, W. Dong and G. Wang, New J. Chem., 2015, 39, 4919 DOI: 10.1039/C5NJ00632E

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