Issue 0, 1975
From the journal:

Journal of the Chemical Society, Faraday Transactions 2: Molecular and Chemical Physics

Theory for time resolved emission spectra

Graham R. Fleming,   Onno L. J. Gijzeman,   Karl F. Freed  and  Sheng H. Lin  

Abstract

Explicit equations for the calculation of time resolved emission spectra from molecules undergoing collisional vibrational relaxation are presented. The equations describe the changes of the emission spectrum with time, after a delta pulse excitation. Alternatively, they can be used to obtain the steady state (frequency resolved) emission spectrum as a function of the pressure of added buffer gas. Some model cases are discussed in the light of available experimental data. Non-monotonic dependences of the emission intensity on time and pressure are exhibited which are related in appearance to those expected from quantum mechanical interference effects.

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Article information

DOI
https://doi.org/10.1039/F29757100773
Article type
Paper

J. Chem. Soc., Faraday Trans. 2, 1975,71, 773-780

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Theory for time resolved emission spectra

G. R. Fleming, O. L. J. Gijzeman, K. F. Freed and S. H. Lin, J. Chem. Soc., Faraday Trans. 2, 1975, 71, 773 DOI: 10.1039/F29757100773

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