Abstract
Chirality, a fundamental concept from biological molecules to advanced materials, is prevalent in nature. Yet, its intricate behavior in specific topological systems remains poorly understood. Here, we investigate the emergence of hidden chiral domain wall states using a double-chain Su-Schrieffer-Heeger model with interchain coupling specifically designed to break chiral symmetry. Our phase diagram reveals single-gap and double-gap phases based on electronic structure, where transitions occur without topological phase changes. In the single-gap phase, we reproduce chiral domain wall states, akin to chiral solitons in the double-chain model, where chirality is encoded in the spectrum and topological charge pumping. In the double-gap phase, we identify hidden chiral domain wall states exhibiting opposite chirality to the domain wall states in the single-gap phase, where the opposite chirality is confirmed through spectrum inversion and charge pumping as the corresponding domain wall slowly moves. By engineering gap structures, we demonstrate control over hidden chiral domain states. Our findings open avenues to investigate novel topological systems with broken chiral symmetry and potential applications in diverse systems.
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Introduction
Chirality and topology are concepts of great importance that lead to novel physical properties and potential applications in various fields. Examples include topological surface states in topological insulators1,2, Majorana fermions in topological superconductors3,4, chiral stacking orders in charge density waves5,6,7, and topological lasers in photonic systems8,9. As prototypical systems, the Su–Schrieffer–Heeger (SSH)10 and Rice-Mele11 models exhibit exotic topological properties such as highly robust Jackiw-Rebbi domain wall zero-energy states12, charge fractionalization13, and spin-charge separation14. As a coupled SSH model, the double-chain (DC) model with broken chiral symmetry shows chiral solitons having topological chiral degrees of freedom and Z4 topological algebraic operation15, where the chirality manifests as a spectrum of the chiral soliton and topological charge pumping observed during the adiabatic process as the chiral soliton slowly moves.
Such SSH and Rice-Mele models have been experimentally realized in various physical systems—polyacetylene10,16, cold atomic systems17,18, artificial electronic lattices19,20, photonic systems21,22, and acoustic systems23,24. Their quantized Berry phases25 are consistent with the bulk-boundary correspondence26,27. While many coupled SSH chain systems with nontrivial topology have been extensively studied28,29,30,31, most possess chiral symmetry, precluding the emergence of chirality as chirality necessitates symmetry breaking. In contrast, the DC model with broken chiral symmetry has been demonstrated in limited physical systems such as self-assembled indium nanowires and artificial atomic chains, exhibiting distinct chiral domain wall states20,32,33. Despite being in the same topological class with preserved time-reversal and broken chiral symmetries15,34,35,36, a comprehensive understanding of such multiband systems remains elusive. Therefore, this work endeavors to present a unified framework elucidating the chirality, topology, and bulk-boundary correspondence underlying the emergence of chiral domain wall states in the coupled SSH chain systems with broken chiral symmetry.
Utilizing a representative DC model with interchain coupling, where chiral symmetry is broken, we unveil the emergence of hidden chiral domain wall states possessing inverted chirality even without necessitating any topological phase transition. Our investigation yields a phase diagram revealing single- and double-gap phases depending on the dimerization of each SSH chain and the strength of the interchain coupling. Within the single-gap phase, the chiral domain wall states manifest as two localized states akin to chiral solitons observed in the DC model32. In the double-gap phase, we observe the emergence of hidden chiral domain wall states characterized by opposite chirality compared to the preexisting domain wall states in the single-gap phase.
We physically verify this opposite chirality through the spectrum inversion of the domain wall state and counter-directional charge pumping observed during the adiabatic process as the domain wall state slowly moves. Using the extended two-dimensional effective Hamiltonian corresponding to the adiabatic process and the Berry curvature distribution, we topologically confirm the chirality of hidden chiral domain wall states. Furthermore, by engineering the gap structure via tuning of the interchain coupling, we successfully control the emergence of the hidden chiral domain state. Our results not only provide insights into the fundamental physics of multiband SSH systems with broken chiral symmetry but also have important implications for the design of novel devices based on chiral domain wall states.
Results and discussion
Double-chain model
First, we introduce the DC model consisting of two SSH chains with interchain coupling (Fig. 1a). The interchain coupling acts as a tuning parameter that controls the electronic structure of this model while it was treated as a small perturbation in the previous works15,32. Combining two SSH Hamiltonians, we get the Hamiltonian of the DC model:
where the spin term is abbreviated. The superscript (i = 1, 2) represents the upper and lower chains. \({c}_{n}^{(i){{{\dagger}}} }\)\(({c}_{n}^{(i)})\) denotes a creation (annihilation) operator for the nth site of the ith chain. \({t}_{n+1,n}^{(i)}=t+{(-1)}^{n+1}{\Delta }^{(i)}\) indicates the horizontal nearest-neighbor hopping integral for the ith chain, where t ( > 0) and Δ(i) represent the hopping amplitude in the absence of dimerization and the energy-valued dimerization displacement of the i-th chain, respectively. α denotes the interchain coupling strength between the lower and upper SSH chains. Since the A and B dimerized states are two degenerate groundstates for each SSH chain, the DC model naturally leads to four degenerate groundstates32, which are denoted as AA, AB, BA, and BB states (Fig. 1a). For instance, the AA groundstate is characterized by Δ(1) = Δ(2) = δ > 0, while the BB groundstate exhibits Δ(1) = Δ(2) = − δ < 0. The DC model is classified into the AI class due to the broken chiral symmetry15,32, while the SSH model belongs to the BDI class due to the preserved time-reversal and chiral symmetries. Such chiral symmetry breaking in the DC model provides the realization of the chirality of the nontrivial domain wall states15,32.
Figure 1b–e shows the calculated phase map as a function of α/t and δ/t and three representative electronic band structures. Depending on the number of gaps, two large distinct regions emerge: single- and double-gap phases (Fig. 1b). Figure 1c shows a single gap between the second and third bands from the bottom, while Fig. 1d, e has an additional gap between the third and fourth bands. Furthermore, the region of the double-gap phase is subdivided into two subregions depending on whether the additional gap is direct or indirect: the upper gap between the red solid and black dashed curves is indirect (Fig. 1d), while the upper gap becomes direct above the black dashed curve (Fig. 1e).
In the SSH model, a one-dimensional one-band metallic chain at half filling undergoes Peierls dimerization, which results in a two-band topological insulator1,37,38. Similarly, the DC model becomes a four-band insulator after the dimerization15,32, which leads to a gap opening between the second and third bands near the Fermi level. On the other hand, the gap-opening mechanism between the third and fourth bands is different due to the strong interchain coupling. As the interchain coupling increases, the energy eigenvalue at kx = 0 of the third band decreases while the energy eigenvalue at kx = π/a0 (a0 is the unit cell size) of the fourth band increases (Fig. 1c–e). Such behavior eventually generates another gap between the third and fourth bands when the interchain coupling is larger than the phase boundary (red line in Fig. 1b). Analytically, the phase boundary between single- and double-gap phases is given by \({\alpha }_{1}=2t+\delta -\sqrt{2{t}^{2}+4t\delta +3{\delta }^{2}}\). Moreover, the system undergoes an indirect-direct gap transition with increasing interchain coupling. The indirect-direct gap transition boundary (dashed line in Fig. 1b) reads as \({\alpha }_{2}=2t-\delta -\sqrt{2{t}^{2}-4t\delta +3{\delta }^{2}}\). Additionally, the inversion symmetry protects the gap-closing between the first and second bands at the Brillouin zone boundary regardless of interchain coupling, the details of which are provided in Supplementary Note 1.
Geometric configurations and quantum spectra of chiral domain walls
We now discuss geometric configurations and quantum energy spectra for all possible domain wall states connecting different groundstates. When two of the four groundstates are connected, we find only three distinct types of geometric configurations for nontrivial domain wall states (inset of Fig. 2a) due to the equivalence between the same geometric configuration of domain walls15,32. To distinguish such nontrivial geometries, we introduce the chirality and denote the AA-BA and AA-AB type configurations as right-chiral (RC) and left-chiral (LC) domain walls, respectively, and the AA-BB type configuration as an achiral (AC) domain wall, following the notation of previous works15,32. For such three geometric configurations of nontrivial domain walls, we obtain the energy spectra and local density of states (LDOS) using tight-binding methods for both single- and double-gap phases (Fig. 2).
Even though the same geometric domain wall configurations are employed for single- and double-gap phases, the electronic features of the localized domain wall states are quite different from each other. In the single-gap phase, only two in-gap states (denoted as ‘2’ and ‘3’ in Fig. 2a, c) exist as localized domain wall states for all three types of domain walls. Two in-gap states for the AA-BA (AA-AB) geometric configuration are located below (above) the midgap, while two in-gap states for the AA-BB geometric configuration are located symmetrically with respect to the midgap. The nontrivial positioning of the localized electronic states of the domain wall results from chiral symmetry breaking32,39. This chiral symmetry breaking confers chirality upon the domain wall states, with chirality being defined by the spectrum and topological charge pumping. These findings shed light on the interplay between chiral symmetry breaking and localized domain wall states, further enriching our understanding of electronic behavior in such systems.
For the double-gap phase (Fig. 2b, d), an additional, otherwise hidden, in-gap state (denoted as ‘4’) emerges in the upper gap, alongside the two in-gap states in the lower gap (denoted as ‘2’ and ‘3’). The two in-gap states of each domain wall in the lower gap appear similar to those in the single-gap phase. Surprisingly, the in-gap state in the upper gap is located oppositely to those in the lower gap for both right- and left-chiral domain walls. To clearly indicate such spectrum inversion of domain wall states between upper and lower gaps with respect to each midgap, we adopt the term ‘chirality inversion’. The chiral inversion also occurs in the achiral AA-BB domain wall even though the in-gap states for the lower and upper gaps seem not to be inverted due to the symmetrical positioning of in-gap states with respect to each midgap. Note that the topological meaning of the chirality inversion is the counter-directional charge pumping observed during the adiabatic process as the domain wall state slowly moves, which will be discussed in the next subsection.
The chirality inversion of the in-gap states of domain walls between the upper and lower gaps becomes more evident when we plot the energy spectra as a function of interchain coupling. Figure 3 shows the evolution of the spectra for domain wall states with increasing interchain coupling, transitioning from the single- to the double-gap phases. Regardless of the interchain coupling, two nontrivial domain wall states always exist in the lower gap. On the other hand, additional domain wall states emerge as the upper gap opens. Even though these additional domain wall states remain hidden in the region of α < α1, they eventually become visible as the upper gap opens in the region of α1 < α < α2. In the region of α ≥ α2 where the upper gap is direct, the emerging domain wall states maintain their relative energy positions within the gap. Therefore, the chirality (or the spectrum feature) of each domain wall state is preserved throughout the evolution.
Before proceeding further, we briefly discuss the states labeled ‘1’ appearing in Figs. 2 and 3. These states are also potential hidden domain wall states between the first and second bands. The LDOS maps in Fig. 2c, d clearly show the localized feature except for the AA-BA configuration in Fig. 2c. In the AA-BA configuration, the domain wall state’s spectrum lies too close to the top of the second band for given parameters, making it hard to distinguish this hidden domain wall state from the bulk state. Moreover, the inversion symmetry protects the gap-closing between the first and second bands at the Brillouin zone boundary, as discussed in the previous subsection (see also Fig. 1). Therefore, the hidden domain wall states labeled ‘1’ cannot manifest as in-gap states. Consequently, we will focus on the other states from now on. However, it is worth noting that the hidden domain wall states labeled ‘1’ can indeed emerge as in-gap states by introducing a symmetry-breaking mechanism that opens up the gap, as demonstrated in Supplementary Fig. 1.
Bulk-boundary correspondence
We now investigate the correspondence between the electronic states and the topological properties of the domain walls using Berry phase and Berry curvature via bulk-boundary correspondence1,2. In the context of one-dimensional systems, the electronic spectra of a domain wall state are related to the Berry phase difference between two groundstates that the domain wall interpolates11,40.
Table 1 shows the calculated Berry phases for the four groundstates up to the second and third bands from the lowest one. The well-separated electronic bands depicted in Fig. 1c–e enable a band-by-band definition of the Berry phase, thereby facilitating a more precise analysis of the system’s electronic and topological properties. All Berry phases are quantized as integer multiples of π/2, due to the Z4 symmetry of the system15,32 (the mathematical details are provided in Supplementary Notes 2 and 3). The Berry phases up to the second band decrease as 0, −π, −2π, and −3π for AA, BA, BB, and AB groundstates. On the other hand, the Berry phases to the third band increase as 0, π/2, π, and 3π/2 for AA, BA, BB, and AB groundstates. In contrast to the SSH model, some Berry phases exceed 2π. It is noteworthy that the Berry phase is defined within a range of modulo 4π instead of the conventional 2π reflecting the evolution of the Wannier center and the Z4 symmetry of the system15,32. Such adjustment also accommodates the charge pumping phenomena occurring during the relevant adiabatic process, as discussed below.
To clarify such Berry phases, as shown in Fig. 4, we plot the continuous change in the Berry phase (or the evolution of the Wannier charge center15,41) up to the second and third bands for three types of cyclic adiabatic processes. These three types of cyclic adiabatic processes are generated when the corresponding types of chiral domain walls move from right to left along the one-dimensional chain. Because there are three types of chiral domain walls, we can identify three distinct cyclic adiabatic processes as follows: (1) RC adiabatic process: AA → BA → BB → AB → AA, (2) LC adiabatic process: AA → AB → BB → BA → AA, and (3) AC adiabatic process: AA → BB → AA.
Above all, we will discuss the Berry phase under RC and LC adiabatic processes. During the RC adiabatic process (Fig. 4a), the total Berry phase up to the second band evolves from 0 to 2π while the one up to the third band changes from 0 to −4π. Conversely, the LC adiabatic process shows the opposite behavior in terms of the Berry phase (Fig. 4b). As a result, two intriguing observations emerge. First, within a given type of adiabatic process, the trends in the Berry phases up to the second and third bands are diametrically opposite. Second, when the chemical potential is held constant, thereby keeping the band occupation constant, the variations in the Berry phases between the RC and LC adiabatic processes are also in opposition. Such findings provide compelling topological evidence for the inversion of chirality between the upper and lower gaps, as well as between RC and LC chiral domain wall states. From a physical perspective, this opposite variation in the Berry phase is tantamount to the counter-directional charge pumping observed during the adiabatic process, which will be elaborated upon in the subsequent paragraph.
From the viewpoint of topology, the chirality of the in-gap state of a domain wall is determined by the direction of topological charge pumping under the adiabatic evolution from one groundstate to the other groundstate when the two groundstates are interpolated by the domain wall11,15,32,34,42. If the direction of topological charge pumping is negative (positive), the electronic states will be located below (above) the midgap. Because the local information of such topological charge pumping is encoded in the Berry curvature during the adiabatic process, we can also identify the chirality of the in-gap state of a domain wall using Berry curvature distribution. Notice that the direction of charge pumping (or the moving direction of the Wannier charge center) and the sign of Berry curvature are inversely related. See more details in Supplementary Note 2.
First, let us consider the in-gap states in the lower gap. For a RC (LC) domain wall connecting AA to BA (AA to AB) groundstates, the sign of Berry curvature distribution up to the second band from the lowest one, as shown in the first (second) panel of Fig. 5b, is positive (negative), and hence, the in-gap states in the lower gap are located below (above) the midgap, as shown in Fig. 3a, b. Thus, the corresponding charge pumping under the RC and LC adiabatic processes are also opposite, as shown in Supplementary Fig. 2.
Next, let us consider the in-gap states in the upper gap. In this case, the directions of topological pumping are reversed compared to those in the lower gap case (Supplementary Fig. 2), which is consistent with the chirality inversion of chiral domain walls between upper and lower gaps. Thus, for a RC (LC) domain wall connecting AA to BA (AA to AB), the sign of the Berry curvature distribution up to the third band in the first (second) panels of Fig. 5a is negative (positive), and hence the in-gap states in the upper gap are located above (below) the midgap as shown in Fig. 3a, b.
Finally, for the in-gap states of AC domain walls in both upper and lower gaps, no charge pumping occurs because of the zero total Berry curvature during the adiabatic process (AA → BB → AA) as shown in the third panels of Fig. 5a, b, which is consistent with the change of the Berry phase in Fig. 4c. This gives the symmetrically located electronic states, as indicated by the purple lines in Fig. 3c.
Note that the same (opposite) Berry curvature distribution is repeated during the chiral (achiral) adiabatic process due to the system’s Z4 symmetry15,32 as shown in Fig. 5, which leads to the quantized Berry phases of the groundstates. Furthermore, we find that the quantized Berry phases for the four groundstates in Table 1 are independent of both interchain coupling and dimerization strength. This strongly implies that both the hidden chiral domain wall state and the in-gap chiral domain wall state possess consistent topological properties, irrespective of the interchain coupling and dimerization. Typically, a topological phase transition occurs when the energy gap between two bands closes and reopens, accompanied by a change in topological invariants. Surprisingly, our study does not observe such a topological transition even after the upper gap opens, as the topological invariants remain unchanged. Note that the structure of Dirac points remains stable regardless of the interchain coupling in the absence of dimerization, as shown in Fig. 6. This observation highlights the robustness of the topological properties in the double-chain model, independent of the interchain coupling.
Conclusion
In summary, we have studied the emergence of the hidden topological domain wall states via gap engineering without requiring any topological phase transition using a representative double-chain SSH model, specifically designed to break the chiral symmetry. By adjusting the dimerization and interchain coupling, we constructed the phase diagram composed of single- and double-gap phases. For a small interchain coupling, we found the chiral domain wall states with two localized in-gap states in the single gap. However, for a larger interchain coupling, hidden domain wall states emerge, featuring only a single localized state in an additional gap. Intriguingly, the chirality of these emergent domain wall states in the second gap was found to be opposite compared to that of the original domain wall states in the first gap. We validated this chirality inversion through spectrum inversion of the domain wall state and the observation of opposite charge pumping during the adiabatic process. The topological confirmation of the chirality of hidden chiral domain wall states was further supported through the analysis of the Berry curvature distribution.
This kind of chirality emergence is plentiful in nature and has many applications such as chirality-dependent light-matter devices43, chiral quantum optics44, and chiral magnetic domain memory devices45,46. Therefore, we expect our theoretical approach can be applied to diverse topological systems such as In/Si(111)32,47, Cl vacancies on Cl/Cu(100)20,33, and photonic lattices as well as topological laser systems8,9. For instance, our model system can be used as a multi-digit topological information carrier39 by engineering the gap structure and Fermi level. We also foresee the possibility of a new type of multi-frequency topological laser, where the topological single-mode lasing frequency can be selectively controlled.
Methods
The band structures and phase diagrams in Figs. 1 and 6 were studied using the Bloch Hamiltonian of the DC model, which is given by
where \({t}_{\pm }^{(i)}=t\pm {\Delta }^{(i)}\) with energy-valued dimerization Δ(i) for the i-th chain.
To obtain the spectra and LDOS for the RC, LC, and AC chiral domain walls states in Figs. 2 and 3, we used the tight-binding method for the finite system having 4n + 3, 4n + 1, and 4n + 2 atoms with n = 200, respectively. Such boundary conditions ensure the absence of localized edge states at both ends. The dimerization patterns for the domain wall states were simulated using the position-dependent dimerizations and hyperbolic tangent functions: \({\Delta }^{(i)}(x)=\pm \delta \tanh (x/\xi )\), with ξ being the characteristic width of the domain wall, where ξ = 1.5a0 in Figs. 2 and 3.
For the Berry phase and Berry curvature in Figs. 4 and 5, we took into account a cyclic adiabatic process of a 1D Hamiltonian, denoted as H(kx, τ), where τ is time for the adiabatic evolution. By extending the 1D lattice system into a 2D lattice system, we replace the time evolution with momentum ky in an extra dimension. Then, we constructed the 2D Hamiltonian H2D(kx, ky) such that H2D(kx, ky = 0) = H(kx, τ = 0) and H2D(kx, ky = 2π) = H(kx, τ = T), where T represents the period of the corresponding cyclic adiabatic process. Using this 2D Hamiltonian, we have calculated the Berry phase and Berry curvature. Further comprehensive information can be found in Supplementary Notes 2–4.
Data availability
The data used in this paper are available from T.-H.K. or S.C. on reasonable request.
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Acknowledgements
This work was supported by the National Research Foundation of Korea (NRF) funded by the Ministry of Science and ICT (MSIT), South Korea (Grants No. NRF-2021R1H1A1013517, NRF-2022R1A2C1011646, NRF-2022M3H3A1085772, NRF-2021R1A6A1A10042944, and 2022M3H4A1A04074153). This work was also supported by Quantum Simulator Development Project for Materials Innovation through the NRF funded by the MSIT, South Korea (Grant No. NRF-2023M3K5A1094813). S.-H.H. and S.C. acknowledge support from the POSCO Science Fellowship of POSCO TJ Park Foundation.
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S.-G.J., T.-H.K., and S.C. conceived and designed the project. S.-G.J. and S.-H.H. performed the tight-binding calculations and analyzed the results under the supervision of T.-H.K. and S.C. All the authors discussed the results and contributed to the writing of the manuscript.
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Jeong, SG., Han, SH., Kim, TH. et al. Revealing inverted chirality of hidden domain wall states in multiband systems without topological transition. Commun Phys 6, 262 (2023). https://doi.org/10.1038/s42005-023-01367-x
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DOI: https://doi.org/10.1038/s42005-023-01367-x
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