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Inelastic Neutron Scattering Studies of First Order Phase Transitions in bcc Solid 4He

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Abstract

We report inelastic neutron scattering studies of the [110] transverse phonon branches of bcc 4He near the bcc-hcp transitions on the solid-liquid coexistence line and near the melting transition. The question behind the experiment was whether these transitions in a quantum solid are in any way different from what one observes in usual materials. In contrast to large softening of the T1 branch seen near the bcc-hcp transition in group IV metals, we found that the transverse phonons in bcc 4He do not soften at all. Altough visual studies of the crystals near the transition are consistent with a martensitic transformation, neutron scattering indicates that the transition in solid 4He is different than in metals. Thus, the mechanism of the bcc-hcp transition remains an open question. Similar study done near the melting transition indicates that none of the phonons measured in the present experiment is affected by melting, which rules out a mechanical instability of the bulk as a mechanism of melting. Finally, in addition to the phonons, we observed a new feature at q=0 and at an energy transfer of 1.23 meV which we attribute to neutron scattering by point defects. Similarly to the phonons, this feature did not change near any of the phase transitions.

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Markovich, T., Polturak, E., Lipson, S.G. et al. Inelastic Neutron Scattering Studies of First Order Phase Transitions in bcc Solid 4He. Journal of Low Temperature Physics 129, 65–77 (2002). https://doi.org/10.1023/A:1020097302352

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