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Rational Design of Nanostructured MnO2 Cathode for High-performance Aqueous Zinc Ion Batteries

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Chemical Research in Chinese Universities Aims and scope

Abstract

Aqueous Zn-MnO2 batteries hold a promising potential for grid-scale energy storage applications due to their intrinsic safety, low fabrication cost, environmental friendliness and high theoretical energy densities. Developing novel nanostructured cathode materials with high discharge voltage, large capacity and excellent structural stability is one of the critical ways to achieve the high-performance aqueous Zn batteries. Enlighten by that, comprehending principles of materials design and identifying the challenges faced by the state-of-the-art MnO2 hosts are vital preconditions. Rather than a simple comparison, this review mainly focuses on design strategies regarding to MnO2-based materials, including defect engineering, interfacial engineering, and pre-intercalation engineering. In addition, the energy storage mechanisms of MnO2-based cathodes are discussed to clarify the complicated chemical reactions during battery cycling. Challenges and perspectives are outlined to guide the further development of advanced Zn-MnO2 batteries.

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Acknowledgements

This work was supported by the National Natural Science Foundation of China (Nos.22209006, 21935001), the Natural Science Foundation of Shandong Province, China (No. ZR2022QE009), the Fundamental Research Funds for the Central Universities of China(No.buctrc202307) and the Key Beijing Natural Science Foundation, China (No. Z210016).

We also thank the Ministry of Finance and the Ministry of Education of China for long-term subsidy mechanism.

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Authors and Affiliations

  1. State Key Laboratory of Chemical Resource Engineering, College of Chemistry, Beijing University of Chemical Technology, Beijing, 100029, P. R. China

    Qi Li, Yajun Zhao, Yueyang Wang, Abdalla Kovan Khasraw, Yi Zhao & Xiaoming Sun

  2. Advanced Technology Research Institute, Beijing Institute of Technology, Jinan, 250300, P. R. China

    Yi Zhao

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  1. Qi Li
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  2. Yajun Zhao
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  3. Yueyang Wang
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  4. Abdalla Kovan Khasraw
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  5. Yi Zhao
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  6. Xiaoming Sun
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Correspondence to Yi Zhao or Xiaoming Sun.

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The authors declare no conflicts of interest.

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Li, Q., Zhao, Y., Wang, Y. et al. Rational Design of Nanostructured MnO2 Cathode for High-performance Aqueous Zinc Ion Batteries. Chem. Res. Chin. Univ. 39, 599–611 (2023). https://doi.org/10.1007/s40242-023-3126-x

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  • DOI: https://doi.org/10.1007/s40242-023-3126-x

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