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High-Temperature Thermal Properties of Ba(Ni1/3Ta2/3)O3 Ceramic and Characteristics of Plasma-Sprayed Coatings

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Abstract

To evaluate its applicability as a ceramic top coat in thermal barrier coatings, Ba(Ni1/3Ta2/3)O3 (BNT) was synthesized by a solid-state reaction method and its phase stability, coefficient of thermal expansion (CTE), and thermal conductivity were measured. Coatings with a structure of plasma-sprayed BNT/yttria-partially stabilized zirconia (YSZ) double ceramic coat and a high-velocity oxygen fuel (HVOF)-sprayed bond coat were fabricated. The thermal shock behavior of the coatings was investigated, and the phase composition and microstructure evolution of the BNT/YSZ coatings were characterized. The results showed that the BNT powder had single perovskite structure that remained unchanged after sintering at 1500 °C for 100 h. The average CTE of the BNT ceramic at 25-1400 °C was found to be 10.2 × 10−6 K−1, comparable to that of YSZ. The thermal conductivity at 1200 °C was found to be 2.56 W m−1 K−1. During thermal shock, the BNT/YSZ coatings spalled layer by layer, which can be attributed to the compositional deviation combined with the large temperature gradient in the BNT coating.

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Acknowledgments

This work was supported by the Natural Science Foundation of Beijing, China (Grant No. 2131006).

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Authors and Affiliations

  1. School of Materials Science and Engineering, Beijing Institute of Technology, Beijing, 100081, China

    Yupeng Cao, Quansheng Wang, Yanbo Liu & Xianjin Ning

  2. National Key Laboratory of Science and Technology on Materials Under Shock and Impact, Beijing, China

    Yupeng Cao, Quansheng Wang, Yanbo Liu & Xianjin Ning

Authors
  1. Yupeng Cao
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  2. Quansheng Wang
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  3. Yanbo Liu
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  4. Xianjin Ning
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Correspondence to Yanbo Liu.

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Cao, Y., Wang, Q., Liu, Y. et al. High-Temperature Thermal Properties of Ba(Ni1/3Ta2/3)O3 Ceramic and Characteristics of Plasma-Sprayed Coatings. J Therm Spray Tech 27, 1594–1601 (2018). https://doi.org/10.1007/s11666-018-0796-x

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  • DOI: https://doi.org/10.1007/s11666-018-0796-x

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