Skip to main content
Log in

Measurement of half-lives for 87m,gY and 196m,g,194Au produced from the photon and neutron induced reactions of 89Y and 197Au

  • Published:
Journal of Radioanalytical and Nuclear Chemistry Aims and scope Submit manuscript

Abstract

We have measured the half-lives of 87mY and 87gY produced from the 89Y(γ, 2n) and 89Y(n, 3n) reactions with the bremsstrahlung end-point energy of 65 MeV and the average neutron energy of 37.2 MeV using an activation and an off-line γ-ray spectrometric technique, respectively. The bremsstrahlung photon was produced by using the 100 MeV electron linac of the Pohang Accelerator Laboratory (PAL), whereas the fast neutron was produced from the 9Be(p, n) reaction by using the 45 MeV proton of the MC-50 Cyclotron at the Korea Institute of Radiological and Medical Sciences (KIRAMS). We have also measured the half-lives of 194Au and 196m2,gAu produced from the 197Au(γ, xn; x = 1, 3) and 197Au(n, xn; x = 2, 4) reactions with the bremsstrahlung end-point energy of 60 MeV and the average neutron energy of 37.2 MeV using the same technique and the same facilities as mentioned above. The induced γ-ray activities of the irradiated samples were measured by using an energy- and efficiency calibrated high purity germanium (HPGe) detector. The spectrum analysis has been done by using the ROOT software to separate signals from background. The measured half-lives are compared with the literature values and are in general agreement with each other within the uncertainties.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Fig. 1
Fig. 2
Fig. 3
Fig. 4
Fig. 5
Fig. 6
Fig. 7
Fig. 8

Similar content being viewed by others

References

  1. Nuttin A, Heuer D, Billebaud A, Brissot R, Le Brun C, Liatard E, Loiseaux JM, Mathieu L, Meplan O, Merle-Lucotte E, Nifenecker H, Perdu F, David S (2005) Proc. Nucl Energy 46:77

    Article  CAS  Google Scholar 

  2. Allen TR, Crawford DC (2007) Sci Technol Nucl Install Article ID 97486

  3. Sinha RK, Kakodkar (2006) Nucl Eng Des 236:683

  4. Carminati F, Klapisch R, Revol JP, Rubio JA, Rubia C (1993) CERN/AT/93-49(ET)

  5. Rubia C, Rubio JA, Buono S, Carminati F, Fietier N, Galvez J, Geles C, Kadi Y, Klapisch R, Man-drilion P, Revol JP, Roche Ch (1997) CERN/LHC/97-01(EET)

  6. Accelerator Driven Systems: Energy Generation and Transmutation of Nuclear Waste, Status report (1997) IAEA, Vienna, IAEA-TECDO-985

  7. Bowman CD (1998) Annu Rev Nucl Part Sci 48:505

    Article  CAS  Google Scholar 

  8. Ganesan S (2007) Pramana 68:257

    Article  CAS  Google Scholar 

  9. Qaim SM (2017) Nucl Med Biol 44:31–49

    Article  CAS  PubMed  Google Scholar 

  10. Escher E, Burke JT, Dietrich FS, Scielzo ND, Ressler JJ (2011) J Phys Conf Ser 322:012006

    Article  CAS  Google Scholar 

  11. Kalamara A, Vlastou R, Kokkoris M, Nicolis NG, Patronis N, Serris M, Michalopoulou V (2018) Phys Rev C 97:034615

    Article  CAS  Google Scholar 

  12. Tsinganis A, Diakaki M, Kokkoris M, Lagoyannis A, Mara E, Papadopoulos CT, Vlastou R (2011) Phys Rev C 83:024609

    Article  CAS  Google Scholar 

  13. Sultan JA, Lauren RL, Valeriia NS (2014) J Radioanal Nucl Chem 302:623–629

    Article  CAS  Google Scholar 

  14. Sokolov AD, Bourmistenko YN, Gostilo VV, Titov VL (2018) Miner Eng 116:179–181

    Article  CAS  Google Scholar 

  15. Daniel SD, Valeriia NS, Tony AF, Emily O (2018) Appl Radiat Isot 139:137–140

    Article  CAS  Google Scholar 

  16. Pillai MRA Yttrium-90 production and radiopharmaceuticals development. https://www.academia.edu/5829195/Chapter_8_Yttrium90_production_and_radiopharmaceuticals_development

  17. Rhman MS, Kim K-S, Lee M, Kim GN, Oh Y, Lee H-S, Cho M-H, Ko IS, Namkung W, Van Do N, Khue PD, Kim TT, Ro T-I (2009) Nucl Instr Meth B 267:3511

    Article  CAS  Google Scholar 

  18. Naik H, Kim GN, Kim K, Zaman M, Sahid M, Yang S-C, Lee MW, Kang YR, Shin SG, Cho M-H, Goswami A, Song TY (2014) J Radioanal Nucl Chem 300:1121

    Article  CAS  Google Scholar 

  19. Tatari M, Kim G, Naik H, Ranjbar AH, Kim K, YangSung C, Zaman M, Shahid M, Shin SG, Gey Y, Cho M (2015) Nucl Instr Meth B 344:76

    Article  CAS  Google Scholar 

  20. Tatari M, Kim GN, Naik H, Kim K, Cho M-H (2017) Radiochim Acta 105:789

    Article  CAS  Google Scholar 

  21. Zaman M, Kim GN, Naik H, Kim K, Shin SG, Cho M-H (2014) J Radioanal Nucl Chem 299:1739

    Article  CAS  Google Scholar 

  22. Zaman M, Kim GN, Kim K, Shahid M, Naik H, Yang SC, Shin SG, Cho M-H (2015) J Korean Phys Soc 67:1482

    Article  CAS  Google Scholar 

  23. Nadeem M, Zaman M, Naik H, Kim K, Kim GN, Shahid M (2018) Nucl Phys A 970:411

    Article  CAS  Google Scholar 

  24. Zaman M, Kim GN, Kim K, Naik H, Lee MW, Nadeem M (2017) Eur Phys J A 53:182

    Article  CAS  Google Scholar 

  25. Zaman M, Kim GN, Naik H, Kim K, Shahid M (2015) J Radioanal Nucl Chem 303:815

    Article  CAS  Google Scholar 

  26. Naik H, Kim GN, Kim K, Zaman M, Goswami A, Lee MW, Yang SC, Lee YO, Shin SG, Cho M-H (2016) Nucl Phys A 948:28

    Article  CAS  Google Scholar 

  27. Weizsacker CF (1934) Z Phys 88:612

    Article  Google Scholar 

  28. Williams EJ (1934) Phys Rev 45:729

    Article  CAS  Google Scholar 

  29. Agostinelli S et al (2005) Nucl Instru Methods A 506:250

    Article  CAS  Google Scholar 

  30. Allison J et al (2006) IEEE Trans Nucl Sci 53:270

    Article  Google Scholar 

  31. Hendricks JS, Gregg WM, Michael LF, Michael RJ, Russell CJ, Joe WD, Joshua PF, Denise, BP, Laurie SW, William WM MCNPX 2.6.0 Extensions, LANL Report LA-UR-08-2216, Los Alamos, 2008. http://mcnpx.lanl.gov/

  32. Zaman M, Kim GN, Kim K, Naik H, Sahid M (2015) Eur Phys J A 51:104

    Article  CAS  Google Scholar 

  33. Brun R, Rademakers F (1997) Nucl Inst Meth A 389:81. https://root.cern.ch/

  34. Morhac M, Kliman J, Matoušek V, Veselsky M, Turzo I (1997) Nucl Inst Meth A 401:113

    Article  CAS  Google Scholar 

  35. NuDat 2.6, National Nuclear Data Center, Brookhaven National Laboratory, updated 2011. http://www.nndc.bnl.gov/

  36. Chu SYF, Ekstrom LP, Firestone RB The Lund/LBNL, Nuclear Data Search, Version 2.0, February 1999, WWW Table of Radioactive Isotopes. http://nucleardata.nuclear.lu.se/toi/

  37. Tanabashi M et al (2018) (Particle Data Group) Phys Rev D 98:30001

Download references

Acknowledgements

The authors would like to express their sincere thanks to the staff of the 100 MeV electron linac of PAL, Pohang and MC-50 Cyclotron in the KIRAMS for the excellent operations and their support during the experiment. This research was supported by the National Research Foundation of Korea through a grant provided by the Ministry of Science, ICT and Future Planning (NRF-2017R1D1A1B03030484, NRF-2018M7A1A1072274, and NRF-2018R1A6A1A06024970).

Author information

Authors and Affiliations

Authors

Corresponding author

Correspondence to Guinyun Kim.

Additional information

Publisher's Note

Springer Nature remains neutral with regard to jurisdictional claims in published maps and institutional affiliations.

Rights and permissions

Reprints and permissions

About this article

Check for updates. Verify currency and authenticity via CrossMark

Cite this article

Jang, W., Zaman, M., Kim, G. et al. Measurement of half-lives for 87m,gY and 196m,g,194Au produced from the photon and neutron induced reactions of 89Y and 197Au. J Radioanal Nucl Chem 321, 765–773 (2019). https://doi.org/10.1007/s10967-019-06629-z

Download citation

  • Received:

  • Published:

  • Issue Date:

  • DOI: https://doi.org/10.1007/s10967-019-06629-z

Keywords

Navigation