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Prompt and delayed inelastic scattering reactions from fission neutron irradiation—first results of FaNGaS

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Abstract

A new instrument for fast neutron gamma spectroscopy has been installed and tested at the Forschungsneutronenquelle Heinz Maier-Leibnitz of the MLZ in Garching. A beam with the flux of about 108 cm−2 s−1 fission neutrons is available to irradiate small samples to study inelastic neutron scattering reactions in materials. A number of relevant elements have been investigated and new gamma lines were identified in comparison to existing data libraries. The method seems to be linear with respect to measurement time and sample mass. A particular advantage of fast neutron PGAA compared to thermal neutron PGAA appears in the analysis of materials with high thermal capture cross sections.

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References

  1. Mauerhofer E, Havenith A (2014) The MEDINA facility for the assey of the chemotoxic inventory of radioactive waste packages. J Radioanal Nucl Chem 302:483–488

    Article  CAS  Google Scholar 

  2. Revay Z, Firestone RB, Molnar GL, Belgya T (2004) In: Molnar G (ed) Handbook of prompt gamma activation analysis with neutron beams. Kluver Academic Publishers, Dordrecht

    Google Scholar 

  3. Ahmed MR, Al-Najjar S, Al-Amili MA, Al-Assafi N, Rammo N, Demidov AM, Govor LI, Cherepantsev YuK (1978) Atlas of gamma-ray spectra from the inelastic scattering of reactor fast neutrons. Atomizdat, Moscow

    Google Scholar 

  4. Plompen AJM, Rouki C, Kopecky S, Krása A, Nankov N, Bacquias A, Dessagne Ph, Kerveno M, Rudolf G, Thiry JC, Borcea C, Negret A, Stanoiu M, Domula A, Zuber K, Angelone M, Pillon M, Hilaire S, Romain P, Archier P, De Saint-Jean C, Noguère G, Koning AJ, Goriely S, Milocco A and Trkov A (2013) Neutron inelastic scattering, recent experiments and their interpretation. In: The 13th international conference on nuclear reaction mechanisms. http://cdsweb.cern.ch/record/1495183 CERN, pp 331–342

  5. Barzilov A, Womble PC (2014) Study of Doppler broadening of gamma-ray spectra in 14-MeV neutron activation analysis. J Radioanal Nucl Chem 301:811–819

    Article  CAS  Google Scholar 

  6. Beyer R, Schwengner R, Hannaske R, Junghans AR, Massarczyk R, Anders M, Bemmerer D, Ferrari A, Hartmann A, Kögler T, Röder M, Schmidt K, Wagner A (2014) Inelastic scattering of fast neutrons from excited states in 56Fe. Nucl Phys A 927:41–52

    Article  CAS  Google Scholar 

  7. Randriamalala T, Rossbach M, Mauerhofer E, Revay Zs, Kudejova P, Söllradl S, Wagner FM, Genreith C (2015) FANGAS: a new instrument for (n,nγ) reaction measurements at FRM II (2015) submitted to Nucl Instr Meth A

  8. Breitkreutz H, Wagner FM, Röhrmoser A, Petry W (2008) Spectral fluence rates of the reactor fast neutron beam MedApp at the FRM II. Nucl Instr Methods A 593:466–471

    Article  CAS  Google Scholar 

  9. Greenwood L, Johnson C (2013) User guide for the STASYL PNNL Suite of Software Tools, PNNL-22253, Pacific Northwest National Laboratory. Richland, Washington 99352

    Book  Google Scholar 

  10. Erdmann G (1976) Neutron activation tables. Verlag Chemie, Weinheim

    Google Scholar 

  11. Yates SW, Filo AJ, Cheng CY, Df Coope (1978) Elemental analysis by gamma-ray detection following inelastic neutron scattering. J Radioanal Nucl Chem 46:343–355

    Article  CAS  Google Scholar 

  12. Ahmed MR, Demidov AM, Al-Najjar SA, Al-Amili MA (1974) Use of spectroscopy of gamma-radiation from the inelastic scattering of reactor fast neutrons for elemental analysis. J Radioanal Nucl Chem 23:199–203

    Article  CAS  Google Scholar 

  13. Randle K (1982) The analytical potential of neutron inelastic scattering reactions. J Radioanal Nucl Chem 72(1–2):405–424

    Article  CAS  Google Scholar 

  14. Randle K (1985) The determination of tungsten in steels by neutron inelastic scattering. J Radioanal Nucl Chem 91(1):185–189

    Article  CAS  Google Scholar 

  15. Castaneda CM, Gearhart R, SanII B, Englert PAJ, Drake DM, Reedy RC (1992) Gamma-ray production cross section from energetic neutron inelastic scattering for methodical improvements in planetary gamma-ray spectroscopy. J Radioanal Nucl Chem 160(2):387–393

    Article  CAS  Google Scholar 

  16. Parsons A, Bodnarik J, Evans L, Floyd S, Lim L, McClanahan T, Namkung M, Nowicki S, Schweizer J, Starr R, Trombka J (2011) Active neutron and gamma-ray instrumentation for in situ planetary science applications. Nucl Instr Meth A 652:674–679

    Article  CAS  Google Scholar 

  17. Filo AJ, Gilbert JW, Yates SW (1979) Simultaneous elemental determination of aluminum and silicone in soil by gamma-ray detection following inelastic neutron scattering. J Radioanal Nucl Chem 54(1–2):235–239

    Article  CAS  Google Scholar 

  18. England TR, Rider BF, LA-UR-94-3106, ENDF-349. http://ie.lbl.gov/fission/238uf.txt. Accessed on 17 Apr 2015

Download references

Acknowledgments

We gratefully acknowledge the help of the FRM II reactor operators and radiation protection staff. This work was financially supported by Bundesministerium für Bildung und Forschung, Germany, grant No. 02S9052A.

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Correspondence to M. Rossbach.

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Rossbach, M., Randriamalala, T., Mauerhofer, E. et al. Prompt and delayed inelastic scattering reactions from fission neutron irradiation—first results of FaNGaS. J Radioanal Nucl Chem 309, 149–154 (2016). https://doi.org/10.1007/s10967-015-4665-5

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  • DOI: https://doi.org/10.1007/s10967-015-4665-5

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