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Ferromagnetism of Mn5Ge3 Precipitates in Mn-implanted Self-organized Ge/Si Quantum Dots

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Abstract

One layer of self-assembled Ge quantum dots with Si barrier were grown on high resistivity (100) p-type Si substrates by rapid thermal chemical vapor deposition followed by Mn ion implantation and post-annealing. A presence of ferromagnetic structure was confirmed in the dilute magnetic quantum dots (DMQD). The DMQD through 10 min annealing was found to be homogeneous, and to exhibit p-type conductivity, insulating property, and ferromagnetic ordering with a Curie temperature, T c=170 K. On the other hand, the DMQD through 30 and 60 min annealing was found to be semi-insulating and ferromagnetic ordering with a Curie temperature over 300 K. The XRD data show that there is a phase separation of Mn rich phases Mn5Ge3 from MnGe nanostructure. Therefore, it is likely that the ferromagnetic exchange coupling of sample with T c=170 K is hole-mediated and the ferromagnetism in sample with T c>300 K is due to Mn5Ge3 phase.

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References

  1. Ohno, H.: Science 281, 951 (1998)

    Article  ADS  Google Scholar 

  2. Dietl, T., Ohno, H., Matsukura, F., Cibert, J., Ferrand, D.: Science 287, 1019 (2000)

    Article  ADS  Google Scholar 

  3. Matsumoto, Y., Murakami, M., Shono, T., Hasegawa, T., Fukumura, T., Kawasaki, M., Ahmet, P., Chihyow, T., Koshihara, S., Koinuma, H.: Science 291, 854 (2001)

    Article  ADS  Google Scholar 

  4. Hartman, T., Lampalzer, M., Klar, P.J., Stolz, W., Heimbrodt, W., Keug von Nidda, H.-A., Loids, A., Svistov, L.: Physica E 13, 572 (2002)

    Article  ADS  Google Scholar 

  5. Theodoropoulou, N., Hebard, A.F., Overberg, M.E., Abernathy, C.R., Pearton, S.J., Chu, S.N.G., Wilson, R.G.: Phys. Rev. Lett. 89, 107203-1 (2002)

    Article  ADS  Google Scholar 

  6. Medvedkin, G.A., Ishibashi, T., Nishi, T., Hayata, K., Hasegawa, Y., Sato, K.: Jpn. J. Appl. Phys. Part 2 39, L949 (2000)

    Article  Google Scholar 

  7. Reed, M.L., El-Masry, N.A., Stadelmaier, H.H., Ritums, M.K., Reed, M.J., Parker, C.A., Roberts, J.C., Bedair, S.M.: Appl. Phys. Lett. 79, 3473 (2001)

    Article  ADS  Google Scholar 

  8. Sonoda, S., Shimizu, S., Sasaki, T., Yamamoto, Y., Hori, H.: J. Cryst. Growth 237–239, 1358 (2002)

    Article  Google Scholar 

  9. Park, Y.D., Hanbicki, A.T., Erwin, S.C., Hellberg, C.S., Sullivan, J.M., Mattson, J.E., Ambrose, T.F., Wilson, A., Spanos, G., Jonker, B.T.: Science 295, 651 (2002)

    Article  ADS  Google Scholar 

  10. Cho, S., Choi, S., Hong, S.C., Kim, Y., Ketterson, J.B., Kim, Y.C., Jung, J.H.: Phys. Rev. B 66, 033303 (2002)

    Article  ADS  Google Scholar 

  11. Chen, J., Wang, K.L., Galatsis, K.: Appl. Phys. Lett. 90, 012501 (2007)

    Article  ADS  Google Scholar 

  12. Zhang, F.M., Liu, X.C., Gao, J., Wu, X.S., Du, Y.W., Zhu, H., Xiao, Q., Chen, P.: Appl. Phys. Lett. 85, 786 (2004)

    Article  ADS  Google Scholar 

  13. Bolduc, M., Awo-Affouda, C., Stollenwerk, A., Huang, M.B., Ramos, F.G., Agnello, G., LaBella, V.P.: Phys. Rev. B 71, 033302 (2005)

    Article  ADS  Google Scholar 

  14. Peressi, M., Debernardi, A., Picozzi, S., Antoniella, F., Continenza, A.: Comput. Mater. Sci. 33, 125 (2005)

    Article  Google Scholar 

  15. Picozzi, S., Antoniella, F., Continenza, A., MoscaConte, A., Debernardi, A., Peressi, M.: Phys. Rev. B 70, 165205 (2004)

    Article  ADS  Google Scholar 

  16. Yu, S.S., Cho, Y.M., Ihm, Y.E., Kim, D.J., Kim, H.J., Hong, S.K., Oh, S.J., Woo, B.C., Kim, C.S.: Curr. Appl. Phys. 6, 478 (2006)

    Article  ADS  Google Scholar 

  17. Stropa, A., Picozzi, S., Continenza, A., Freeman, A.J.: Phys. Rev. B 68, 155203 (2003)

    Article  ADS  Google Scholar 

  18. Yamada, N., Maeda, K., Usami, Y., Ohoyama, T.: J. Phys. Soc. Jpn. 55, 3721 (1986)

    Article  ADS  Google Scholar 

  19. Holub, M., Chakrabarti, S., Fathpour, S., Bhattacharya, P., Lei, Y., Ghosh, S.: Appl. Phys. Lett. 85, 973 (2004)

    Article  ADS  Google Scholar 

  20. Ashcroft, M.W., Mermin, N.D.: Solid State Physics. Saunders College, Philadelphia (1976)

    Google Scholar 

  21. Kittel, C.: Introduction to Solid State Physics. Wiley, New York (1996)

    Google Scholar 

  22. Sarma, S.D., Hwang, E.H., Kaminski, A.: Phys. Rev. B 67, 155201 (2003)

    Article  ADS  Google Scholar 

  23. Woodbury, H.H., Tyler, W.W.: Phys. Rev. 100, 659 (1955)

    Article  ADS  Google Scholar 

  24. Bihler, C., Jaeger, C., Vallaitis, T., Gjukic, M., Brandt, M.S., Pippel, E., Woltersdorf, J., Gösele, U.: Appl. Phys. Lett. 88, 112506 (2006)

    Article  ADS  Google Scholar 

  25. Chen, J., Wang, K.L., Galatsis, K.: Appl. Phys. Lett. 90, 012501 (2007)

    Article  ADS  Google Scholar 

  26. Morresi, L., Pinto, N., Ficcadenti, M., Murri, R., D’Orazio, F., Lucari, F.: Mater. Sci. Eng. B 126, 197 (2006)

    Article  Google Scholar 

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Yoon, I.T. Ferromagnetism of Mn5Ge3 Precipitates in Mn-implanted Self-organized Ge/Si Quantum Dots. J Supercond Nov Magn 23, 319–323 (2010). https://doi.org/10.1007/s10948-009-0532-3

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  • DOI: https://doi.org/10.1007/s10948-009-0532-3

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