Abstract
Efficient ternary organic solar cells were achieved by utilizing an ultra-narrow bandgap material, IEICO-4 F, mixed with the fullerene material PC71BM as the acceptor and PTB7-Th polymer as the donor. The different weights of IEICO-4 F were dropped into the active layer to adjust the ratio of acceptor and donor, optimizing the performance of the cells. The results showed the ternary organic solar cells with 10wt% IEICO-4 F could obtain a higher short-circuit current density resulting in the power conversion efficiency (PCE) up to 9.56%. MoO3/Ag/MoO3 as the transparent electrodes of the semitransparent organic solar cell (ST-OSCs) were prepared. The different thicknesses of Ag impacts on the performance of the ST-OSCs were investigated. The PCE of the ternary ST-OSCs was increased to 7.34% and the average visible light transmittance (AVT) was increased to 28.74% when Ag was 10 nm thickness. The ternary ST-OSCs presented both a good light transmittance and a high PCE. In addition, the light utilization efficiency of the ST-OSCs was increased to 2.1%, and the color reproduction index was improved too. The PCE and AVT of the ST-OSCs could improve simultaneously due to the appropriate ratio of the acceptor and donor as well as the optimized transparent electrodes.
Similar content being viewed by others
Data availability
Can be provided when necessary.
References
W.B. Tarique, A. Uddin et al., Mat. Sci. Semicon Proc. (2023). https://doi.org/10.1016/j.mssp.2023.107541
A. Colsmann, H. Roehm, C. Sprau et al., Sol. RRL (2020). https://doi.org/10.1002/solr.202000015
M. Riede, D. Spoltore, K. Leo et al., Adv. Eng. Mater. (2021). https://doi.org/10.1002/aenm.202002653
J. Miao, F. Zhang, M. Du, W. Wang, Y. Fang et al., Adv. Opt. Mater. (2018). https://doi.org/10.1002/adom.201800001
H. Kang, G. Kim, J. Kim, S. Kwon, H. Kim, K. Lee et al., Adv. Mater. 28, 7821–7861 (2016). https://doi.org/10.1002/adma.201601197
C. Xie, Y. Liu, W. Wei, Y. Zhou et al., Adv. Funct. Mater. (2023). https://doi.org/10.1002/adfm.202210675
G. Zeng, J. Zhang, X. Chen, H. Gu, Y. Li, Y. Li et al., Sci. China Chem. 62, 851–858 (2019). https://doi.org/10.1007/s11426-018-9430-8
E. Muchuweni, E.T. Mombeshora, B.S. Martincigh, V.O. Nyamori et al., Front. Chem. (2022). https://doi.org/10.3389/fchem.2021.733552
E. Ravishankar, R.E. Booth, C. Saravitz, H. Sederoff, H.W. Ade, B.T. O’Connor et al., Joule. 4, 490–506 (2020). https://doi.org/10.1016/j.joule.2019.12.018
S. Han, Y. Deng, W. Han, G. Ren, Z. Song, C. Liu, W. Guo et al., Sol. Energy 225, 97–107 (2021). https://doi.org/10.1016/j.solener.2021.06.068
Y. Zhao, Y. Zhu, H.-W. Cheng, R. Zheng, D. Meng, Y. Yang et al., Mater. Today Energy (2021). https://doi.org/10.1016/j.mtener.2021.100852
L. Zheng, M. Li, S. Dai, Y. Wu, Y. Cai, X. Zhu, S. Ma, D. Yun, J.-F. Li et al., J. Phys. Chem. C 125, 18623–18629 (2021). https://doi.org/10.1021/acs.jpcc.1c05736
K. Yu, W. Song, J. Ge, K. Zheng, L. Xie, Z. Chen, Y. Qiu, L. Hong, C. Liu, Z. Ge et al., Sci. China Chem. 65, 1615–1622 (2022). https://doi.org/10.1007/s11426-022-1270-5
X. Liu, Z. Liu, M. Chen, Q. Wang, F. Pan, H. Liu, L. Zhang, J. Chen et al., Macromol. Rapid Comm. (2022). https://doi.org/10.1002/marc.202200199
X. Huang, J. Oh, Y. Cheng, B. Huang, S. Ding, Q. He, F. Wu, C. Yang, L. Chen, Y. Chen et al., J. Mater. Chem. A 9, 5711–5719 (2021). https://doi.org/10.1039/d0ta11203h
Z. Hu, J. Wang, Z. Wang, W. Gao, Q. An, M. Zhang, X. Ma, J. Wang, J. Miao, C. Yang et al., Nano Energy. 55, 424–432 (2019). https://doi.org/10.1016/j.nanoen.2018.11.010
X. Ma, Z. Xiao, Q. An, M. Zhang, Z. Hu, J. Wang, L. Ding, F. Zhang et al., J. Mater. Chem. A 6, 21485–21492 (2018). https://doi.org/10.1039/c8ta08891h
Y. Xie, L. Huo, B. Fan, H. Fu, Y. Cai, L. Zhang, Z. Li, Y. Wang, W. Ma, Y. Chen et al., Adv. Funct. Mater. (2018). https://doi.org/10.1002/adfm.201800627
S.J. Jeon, Y.C. Kim, J.Y. Kim, J.H. Kim, N.G. Yang, Y.J. Lee, H.S. Lee, Y.H. Kim, G.W. Kim, E.M. Jang et al., Chem. Eng. J. (2023). https://doi.org/10.1016/j.cej.2023.144850
J. He, Q. Zheng, Z. Ren, J. Yu, H. Deng, Y. Lai, S. Cheng et al., Sol. Energy 220, 394–399 (2021). https://doi.org/10.1016/j.solener.2021.03.075
Q. Zheng, P.-S. Chen, J.-G. Huang, S.-L. Du, H. Zhou, H. Deng, C.-X. Zhang, J.-H. Wu, S.-Y. Cheng et al., J. Mater. Sci. Mater. (2023). https://doi.org/10.1007/s10854-022-09705-5
Q. Zheng, S. Du, Q. Sun, J. Huang, P. Chen, H. Zhou, H. Deng, C. Zhang, J. Wu, S. Cheng et al., J. Mater. Sci-Mater. El. (2023). https://doi.org/10.1007/s10854-023-10590-9
Q. Zheng, J. Huang, P. Chen, S. Du, H. Zhou, Q. Sun, H. Deng, J. Wu, C. Zhang, S. Cheng et al., Appl. Phys. Mater. (2023). https://doi.org/10.1007/s00339-023-06533-0
X. Li, X. Liu, W. Zhang, H.-Q. Wang, J. Fang et al., Chem. Mater. 29, 4176–4180 (2017). https://doi.org/10.1021/acs.chemmater.7b01615
J.C. Blakesley, F.A. Castro, W. Kylberg, G.F.A. Dibb, C. Arantes, R. Valaski, M. Cremona, J.S. Kim, J.-S. Kim et al., Org. Electron. 15, 1263–1272 (2014). https://doi.org/10.1016/j.orgel.2014.02.008
A. Melianas, V. Pranculis, Y. Xia, N. Felekidis, O. Inganas, V. Gulbinas, M. Kemerink et al., Adv. Eng. Mater. (2017). https://doi.org/10.1002/aenm.201602143
D. Krisztian, F. Korsos, G. Havasi et al., Sol. Energy Mater. Sol. Cells (2023). https://doi.org/10.1016/j.solmat.2023.112461
M. Zhang, F. Zhang, Q. An, Q. Sun, W. Wang, J. Zhang, W. Tang et al., Nano Energy. 22, 241–254 (2016). https://doi.org/10.1016/j.nanoen.2016.02.032
S.K. Pal, T. Kesti, M. Maiti, F. Zhang, O. Inganas, S. Hellstrom, M.R. Andersson, F. Oswald, F. Langa, T. Osterman et al., J. Am. Chem. Soc. 132, 12440–12451 (2010). https://doi.org/10.1021/ja104786x
X. Ma, F. Zhang, Q. An, Q. Sun, M. Zhang, J. Miao, Z. Hu, J. Zhang et al., J. Mater. Chem. A 5, 13145–13153 (2017). https://doi.org/10.1039/c7ta03472e
Funding
This study was funded by the National Natural Science Foundation of China (No. 61704028, No. 52372183), and the young and middle-aged teacher education research project of Fujian Provincial Department of Education (JAT220011).
Author information
Authors and Affiliations
Contributions
All authors contributed to the study conception and design. Material preparation, data collection, and analysis were performed by [HZ], [PC], [JH], and [SD]. The first draft of the manuscript was written by [QZ] and all authors commented on previous versions of the manuscript. All authors read and approved the final manuscript.
Corresponding author
Ethics declarations
Conflict of interest
The authors declare that they have no known competing financial interests or personal relationships that could have appeared to influence the work reported in this paper.
Additional information
Publisher’s Note
Springer Nature remains neutral with regard to jurisdictional claims in published maps and institutional affiliations.
Rights and permissions
Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law.
About this article
Cite this article
Zheng, Q., Zhou, H., Du, S. et al. Efficiency and average visible light transmittance improved simultaneously of the semitransparent organic solar cells. J Mater Sci: Mater Electron 35, 384 (2024). https://doi.org/10.1007/s10854-024-12167-6
Received:
Accepted:
Published:
DOI: https://doi.org/10.1007/s10854-024-12167-6