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Conductive mechanism and the enhancement high-power electrical properties of Mn-modified Bi(Sc3/4In1/4)O3–PbTiO3–Pb(Mg1/3Nb2/3)O3 high temperature piezoelectric ceramics

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Abstract

In this research, we report the improved high-power electrical properties and the conductive mechanism of the 0.40Bi(Sc3/4In1/4)O3–0.58PbTiO3–0.02Pb(Mg1/3Nb2/3)O3–xMnO2 (BSI–PT–PMN–xMn, x = 0.0–0.8) system synthesized by a modified two-step solid state reaction method. A pure perovskite phase has been detected by the X-ray diffraction analysis of the BSI–PT–PMN–xMn ceramics, and the mechanical quality factor Qm has been found to increase from 28 to 210 with Mn content increasing from 0.0 to 0.8. The DC resistivity measurement indicated that the resistivity of the BSI–PT–PMN–xMn ceramics increases firstly, reaching the maximum at x = 0.4, and then decreases with more Mn modified. The conduction behavior can be described by the intrinsic charge carriers conduction mechanism and extrinsic semiconductor conductive mechanism in different temperature range. The high DC resistivity over 109 Ω cm at 300 °C together with the good electrical properties of piezoelectric constant d33 336 pC/N, planar electromechanical coupling factor kp 42.8%, mechanical quality factor Qm 120 and Curie temperature Tc 414 °C of the BSI–PT–PMN–0.4Mn ceramics makes it promising candidates for high temperature high-power piezoelectric applications.

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Acknowledgements

This work was supported by the Fundamental Research Funds for the Central Universities (Grant Nos. XJS17026, JBX171106), the National Natural Science Foundations of China (Grant No. 51802242), and the 111 Project (No. B12026).

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Author notes

  1. Lei Wang and Tian-Long Zhao have contributed equally to this work.

Authors and Affiliations

  1. School of Microelectronics, Xidian University, Xi’an, 710071, China

    Lei Wang, Tian-Long Zhao, Xianying Dai & Jianjun Song

  2. Department of Materials Science and Engineering, College of Engineering, Peking University, Beijing, 100871, China

    Shuxiang Dong

Authors
  1. Lei Wang
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  2. Tian-Long Zhao
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  3. Xianying Dai
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Correspondence to Xianying Dai or Shuxiang Dong.

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Wang, L., Zhao, TL., Dai, X. et al. Conductive mechanism and the enhancement high-power electrical properties of Mn-modified Bi(Sc3/4In1/4)O3–PbTiO3–Pb(Mg1/3Nb2/3)O3 high temperature piezoelectric ceramics. J Mater Sci: Mater Electron 30, 7780–7786 (2019). https://doi.org/10.1007/s10854-019-01093-7

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  • DOI: https://doi.org/10.1007/s10854-019-01093-7

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