Abstract
Identifying the current pollution status, future trends, and driving factors is a crucial prerequisite for protecting and managing soil environmental quality in light of the challenging soil heavy metal pollution situation. In this study, a typical industrial city in southeast China was selected as the study area. The environmental capacity of 12 heavy metals was first measured for the evaluation of soil heavy metal pollution, and then spatiotemporal change was simulated using indicator Kriging to warn the pollution risk. Finally, the driving factors of heavy metal pollution were analyzed using random forest and geographical detectors. The results revealed that the average environmental capacity index was 0.768, at a medium capacity level. The environmental capacity of each heavy metal showed a decreasing trend from 2016 to 2035. In 2035, the dynamic environmental capacity of each heavy metal element will have decreased by more than 75% if no preventative and remedial measures are taken. The distance from rivers, fine particulate matter, organic matter content, population density, and distance from industrial enterprises were the main factors contributing to heavy metal pollution in soil. The interaction effect of two environmental factors will mostly lead to the intensification of pollution. Based on the results, this study discussed strategies for controlling and remediating the polluted land. These findings could support the source investigation and early warning of soil heavy metal pollution, which are crucial to manag soil pollution and alleviating environmental quality issues.
Similar content being viewed by others
Data availability
The datasets used and/or analyzed during the current study are available from the corresponding author reasonable request.
References
Argyropoulos G, Samara C (2011) Development and application of a robotic chemical mass balance model for source apportionment of atmospheric particulate matter. Environ Model Softw 26(4):469–481
Askari MS, Alamdari P, Chahardoli S, Afshari A (2020) Quantification of heavy metal pollution for environmental assessment of soil condition. Environ Monit Assess 192(3):1–7
Chen J, Bi J, Wu J, Yang G (2011) Prediction of the trend for soil pollution of heavy metals in soils at Huzhou and Evaluation of the environmental capacity. Earth Environ 39(4):531–535
Chen T, Chang Q, Clevers JGPW, Kooistra L (2015) Rapid identification of soil cadmium pollution risk at regional scale based on visible and near-infrared spectroscopy. Environ Pollut 206:217–226
Chen T, Chang Q, Liu J, Clevers JGPW, Kooistra L (2016) Identification of soil heavy metal sources and improvement in spatial mapping based on soil spectral information: a case study in northwest China. Sci Total Environ 565:155–164
Chen Y, Wang W, Shi H, Wang M, Xu C (2019a) Comparative case study on the influence of spatial distribution of heavy metals in regional area. Res Environ Sci 32(7):1213–1223
Chen Y, Weng L, Ma J, Wu X, Li Y (2019b) Review on the last ten years of research on source identification of heavy metal pollution in soils. J Agro Environ Sci 38(10):2219–2238
Chen BY, Liu KL, Liu YL, Qin J, Peng ZH (2021) Source identification, spatial distribution pattern, risk assessment and influencing factors for soil heavy metal pollution in a high-tech industrial development zone in Central China. Hum Ecol Risk Assess 27(2):560–574
Chen H, Wang L, Hu B, Xu J, Liu X (2022) Potential driving forces and probabilistic health risks of heavy metal accumulation in the soils from an e-waste area, southeast China. Chemosphere 289:133182
Eid EM, Galal TM, El-Bebany AF (2020) Prediction models for monitoring heavy-metal accumulation by wheat (Triticum aestivum L.) plants grown in sewage sludge amended soil. Int J Phytoremediat 22(10):1000–1008
Fan Y, Wang Y (2009) Background characteristics of soil elementsin four plains of zhejiang province. Geophys Geochem Explor 33(2):132–134
Fan M, Yang H, Huang X, Cao R, Zhang Z, Hu J, Qin F (2016) Chemical forms and risk assessment of heavy metals in soils around a typical coal-fired power plant located in the mountainous area. China Environ Sci 36(8):2425–2436
Fu C, Wang W, Pan J, Lu H, Liao Q (2014) Research of heavy metal environmental capacity in Lishui District. Nanjing Chin J Soil Sci 45(3):734–742
Gan Y, Huang X, Li S, Liu N, Li YC, Freidenreich A, Wang W, Wang R, Dai J (2019) Source quantification and potential risk of mercury, cadmium, arsenic, lead, and chromium in farmland soils of Yellow River Delta. J Clean Prod 221:98–107
Guan Q, Zhao R, Pan N, Wang F, Yang Y, Luo H (2019) Source apportionment of heavy metals in farmland soil of Wuwei, China: comparison of three receptor models. J Clean Prod 237:117792
He M, Yan P, Yu H, Yang S, Xu J, Liu X (2020) Spatiotemporal modeling of soil heavy metals and early warnings from scenarios-based prediction. Chemosphere 255:126908
Hou D, O’Connor D, Igalavithana AD, Alessi DS, Luo J, Tsang DCW, Sparks DL, Yamauchi Y, Rinklebe J, Ok YS (2020) Metal contamination and bioremediation of agricultural soils for food safety and sustainability. Nat Rev Earth Environ 1(7):366–381
Jiang YF, Guo X (2019) Multivariate and geostatistical analyses of heavy metal pollution from different sources among farmlands in the Poyang Lake region. China J Soils Sedim 19(5):2472–2484
Jiang H, Wang C, Bai L, Han C, Chen X, Wang C (2020) Advances and prospects in lake environment science and engineering: a review. Hupo Kexue 32(5):1278–1296
Jiang Y, You Q, Chen X, Jia X, Xu K, Chen Q, Chen S, Hu B, Shi Z (2022) Preliminary risk assessment of regional industrial enterprise sites based on big data. Sci the Total Environ 838:156609
Li Y, Han P, Ren D, Luo N, Wang J (2017) Influence factor analysis of farmland soil heavy metal based on the geographical detector. Sci Agric Sin 50(21):4138–4148
Li X, Cundy AB, Chen W, Liu R, Lv S (2020) Dynamic capacity modelling of soil environment carrying capacity, and developing a soil quality early warning framework for development land in China. J Clean Prod 257:120450
Li X, Geng T, Shen W, Zhang J, Zhou Y (2021) Quantifying the influencing factors and multi-factor interactions affecting cadmium accumulation in limestone-derived agricultural soil using random forest (RF) approach. Ecotoxicol Environ Saf 209:111773
Liang F, Pan Y, Peng H, Zeng M, Huang C (2022) Time-space simulation, health risk warning and policy recommendations of environmental capacity for heavy metals in the pearl river Basin, China. Int J Environ Res Public Health 19(8):4694
Lin Y-P, Cheng B-Y, Shyu G-S, Chang T-K (2010) Combining a finite mixture distribution model with indicator kriging to delineate and map the spatial patterns of soil heavy metal pollution in Chunghua County, central Taiwan. Environ Pollut 158(1):235–244
Liu P, Wu K, Luo M (2020) Potential risk factors identification of heavy metals spatial variation in typical agricultural land topsoil of Taihu Basin. Resour Environ Yangtze Basin 29(3):609–622
Liu X, Chen S, Yan X, Liang T, Yang X, El-Naggar A, Liu J, Chen H (2021) Evaluation of potential ecological risks in potential toxic elements contaminated agricultural soils: correlations between soil contamination and polymetallic mining activity. J Environ Manag 300:113679
Lu Q, Wang S, Bai X, Liu F, Li C, Deng Y, Tian S (2021) Quantitative assessment of human health risks under different land uses based on soil heavy metal pollution sources. Hum Ecol Risk Assess 27(2):327–343
Lv Y, Xie L, Zhu W, Zhou Y, Sun H (2020) Risk prediction of heavy metals in farmland soil based on environmental capacity: case study of the county scale in Northern Zhejiang Province. Resour Environ Yangtze Basin 29(1):253–264
Obiora SC, Chukwu A, Davies TC (2016) Heavy metals and health risk assessment of arable soils and food crops around Pb-Zn mining localities in Enyigba, southeastern Nigeria. J Afr Earth Sc 116:182–189
Pan YJ, Ding L, Xie SY, Zeng M, Zhang J, Peng HX (2021) Spatiotemporal simulation, early warning, and policy recommendations of the soil heavy metal environmental capacity of the agricultural land in a typical industrial city in China: Case of Zhongshan City. J Clean Prod 285:124849
Qu M, Li W, Zhang C, Wang S, Yang Y, He L (2013) Source apportionment of heavy metals in soils using multivariate statistics and geostatistics. Pedosphere 23(04):437–444
Shao W, Guan Q, Tan Z, Luo H, Li H, Sun Y, Ma Y (2021) Application of BP - ANN model in evaluation of soil quality in the arid area, northwest China. Soil Tillage Res 208:104907
Shen TL, Liu L, Li YC, Wang Q, Dai JL, Wang RQ (2019) Long-term effects of untreated wastewater on soil bacterial communities. Sci Total Environ 646:940–950
Shi T, Hu Z, Shi Z, Guo L, Chen Y, Li Q, Wu G (2018) Geo-detection of factors controlling spatial patterns of heavy metals in urban topsoil using multi-source data. Sci Total Environ 643:451–459
Six L, Smolders E (2014) Future trends in soil cadmium concentration under current cadmium fluxes to European agricultural soils. Sci Total Environ 485:319–328
Tan K, Wang H, Chen L, Du Q, Du P, Pan C (2020) Estimation of the spatial distribution of heavy metal in agricultural soils using airborne hyperspectral imaging and random forest. J Hazard Mater 382:120987
Tian K, Li M, Hu W, Fan Y, Huang B, Zhao Y (2022) Environmental capacity of heavy metals in intensive agricultural soils: Insights from geochemical baselines and source apportionment. Sci Total Environ 819:153078
Vicente AB, Jordan MM, Sanfeliu T, Sanchez A, Esteban MD (2012) Air pollution prediction models of particles, As, Cd, Ni and Pb in a highly industrialized area in Castellon (NE, Spain). Environ Earth Sci 66(3):879–888
Wang J, Xu C (2017) Geodetector: principle and prospective. Acta Geogr Sin 72(1):116–134
Wang J-F, Li X-H, Christakos G, Liao Y-L, Zhang T, Gu X, Zheng X-Y (2010) Geographical detectors-based health risk assessment and its application in the neural tube defects study of the Heshun Region, China. Int J Geogr Inf Sci 24(1):107–127
Wang S, Cai L-M, Wen H-H, Luo J, Wang Q-S, Liu X (2019) Spatial distribution and source apportionment of heavy metals in soil from a typical county-level city of Guangdong Province, China. Sci Total Environ 655:92–101
Wang H, Yilihamu Q, Yuan M, Bai H, Xu H, Wu J (2020) Prediction models of soil heavy metal(loid)s concentration for agricultural land in Dongli: a comparison of regression and random forest. Ecol Indic 119:106801
Wang YZ, Duan XJ, Wang L (2020) Spatial distribution and source analysis of heavy metals in soils influenced by industrial enterprise distribution: case study in Jiangsu Province. Sci Total Environ 710:134953
Wang S, Zhang Y, Cheng J, Li Y, Li F, Li Y, Shi Z (2022) Pollution assessment and source apportionment of soil heavy metals in a coastal industrial city, Zhejiang, Southeastern China. Int J Environ Res Public Health 19(6):3335
Wu X, Huang X, Li C, Hu J, Tang F, Zhang Z (2018) Soil heavy metal pollution degrees and metal chemical forms around the coal mining area in Western Guizhou. Res Soil Water Conserv 25(6):335–341
Xia X, Yang Z, Cui Y, Li Y, Hou Q, Yu T (2014) Soil heavy metal concentrations and their typical input and output fluxes on the southern Song-nen Plain, Heilongjiang Province, China. J Geochem Explor 139:85–96
Yan N, Liu W, Xie H, Gao L, Han Y, Wang M, Li H (2016) Distribution and assessment of heavy metals in the surface sediment of Yellow River. China J Environ Sci 39(01):45–51
Yan T, Zhao W, Yu X, Li H, Gao Z, Ding M, Yue J (2022) Evaluating heavy metal pollution and potential risk of soil around a coal mining region of Tai’an City. China Alex Eng J 61(3):2156–2165
Yu G, Cheng J, Wang Z, Mu J, Jing L (2009) Soil-environmental capacity in different vegetative types in Shandong province. J Soil Sci 40(2):366–368
Zhang G, Wu H (2018) From problems to solutions: soil functions for realization of sustainable development goals. Bull Chin Acad Sci 33(2):124–134
Zhang J, Xie G, Sun H (2016) Evaluation of soil heavy metal pollution of geological anomaly area based on improved fuzzy comprehensive evaluation methodA case study of Guannan in Jiangsu Province. China J Agro Environ Sci 35(11):2107–2115
Zhang K, Yang J, Ji Y, Xia Y (2018) Spatiotemporal simulation and predication of heavy metal(loid) concentrations in coal chemical industrial areas with a soil environmental capacity model. Int J Coal Sci Technol 5:508–518
Zhang B, Liu L, Huang Z, Hou H, Zhao L, Sun Z (2021) Application of stochastic model to assessment of heavy metal(loid)s source apportionment and bio-availability in rice fields of karst area. Sci Total Environ 793:148614
Zhao Y, Tang S, Li Y, Shi R, Ju X, Wang R (2009) Application of ordinary and indicator Kriging methods for screening non-rice-cropping areas. Acta Sci Circum 29(8):1780–1787
Zhou X, Wang X (2019) Impact of industrial activities on heavy metal contamination in soils in three major urban agglomerations of China. J Clean Prod 230:1–10
Acknowledgements
This work was founded by The Natural Science Foundation of Zhejiang Province (No.LZ21D010002); the Key Research and Development Program of Zhejiang Province (2023C03134); the Zhejiang Province Public Welfare Technology Application Research Project (LGN22D010003); and the National Natural Science Foundation of China (No.41771244)
Funding
This work was supported by the Natural Science Foundation of Zhejiang Province (LZ21D010002); the Key Research and Development Program of Zhejiang Province (2023C03134); the Zhejiang Province Public Welfare Technology Application Research Project (LGN22D010003); and the National Natural Science Foundation of China (41771244).
Author information
Authors and Affiliations
Contributions
JM: Conceptualization, formal analysis, writing—original draft, writing—review and editing. KL: Methodology, software, visualization. YL: Conceptualization, data curation, writing—review and editing. YZ: Investigation, validation. FL, FX: Project administration, supervision, validation. YL: Project administration, resources, supervision, validation. All authors commented on previous versions of the manuscript. All authors read and approved the final manuscript.
Corresponding author
Ethics declarations
Conflict of interest
The authors have no relevant financial or non-financial interests to disclose.
Additional information
Publisher's Note
Springer Nature remains neutral with regard to jurisdictional claims in published maps and institutional affiliations.
Rights and permissions
Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law.
About this article
Cite this article
Ma, J., Lei, K., Li, Y. et al. Spatiotemporal simulation, early warning, and driving factors of soil heavy metal pollution in a typical industrial city in southeast China. Stoch Environ Res Risk Assess 38, 315–337 (2024). https://doi.org/10.1007/s00477-023-02581-3
Accepted:
Published:
Issue Date:
DOI: https://doi.org/10.1007/s00477-023-02581-3