Abstract
Multipass cells (MPC) have been widely used for high-sensitivity spectroscopic measurements. We report the linear scalability in the configuration design of an MPC, which is derived from ray transfer equations in the non-paraxial approximation. As a proof of principle, twelve sets of Herriot-type cells ranging from 4.6 × 4.6 × 12.3 to 57.1 × 57.1 × 147.7 mm3 were investigated with their beam patterns and optical path lengths modeled. By taking the non-intersecting seven-circle beam pattern as a typical example, the designated beam patterns were successfully reproduced by modeling and the optical path length scales linearly with the cell size. Two sets of MPCs were also fabricated by additive manufacturing to further justify the rationale of linear scalability. Possible effects of beam spot size and the signal-to-noise ratio on the miniaturization and escalation of MPCs were discussed. This work contributes to a new insight into the cell configuration and will be useful for accelerating the cell design at various scales.
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The data that support the findings of this study are available from the corresponding authors upon reasonable request.
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Acknowledgements
This work is supported by National Natural Science Foundation of China (52206070), Venture & Innovation Support Program for Chongqing Overseas Returnees (cx2021080), Innovative Research Group Project of National Natural Science Foundation of China (52021004), GROTESK—Generative Fertigung optischer, thermaler und struktureller Komponenten", funded by EFRE—NBank (ZW6-85018307) and Cluster of Excellence PhoenixD (EXC 2122, Project ID 390833453) funded by the Deutsche Forschungsgemeinschaft (DFG, German Research Foundation) within Germany’s Excellence Strategy. We thank Prof. Liu Kun at Anhui Institute of Optics and Fine Mechanics, Chinese Academy of Sciences for help in the MPC alignment.
Funding
Innovative Research Group Project of the National Natural Science Foundation of China, 52021004, National Natural Science Foundation of China, 52206070, Venture & Innovation Support Program for Chongqing Overseas Returnees, cx2021080, EFRE-NBank, ZW6-85018307, Deutsche Forschungsgemeinschaft, 390833453.
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Junjun proposed the idea, conducted theoretical analysis, and wrote the main manuscript text; Tobias designed the experiment, conducted the modeling, and also wrote part of the manuscript; Jan-Luca & Joshua conducted the experiments and implemented the modeling; The rest authors have helped or participated in the discussion and provided very useful suggestions to improve this work; All authors reviewed the manuscript.
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Wu, J., Grabe, T., Götz, JL. et al. Linear scalability of dense-pattern Herriott-type multipass cell design. Appl. Phys. B 129, 87 (2023). https://doi.org/10.1007/s00340-023-08031-w
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DOI: https://doi.org/10.1007/s00340-023-08031-w