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Compositional induced structural, dielectric, ferroelectric and optical study of Bismuth modified Barium Titanate ceramic

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Abstract

The present manuscript reports the structural, dielectric, ferroelectric and optical properties of Bi substituted BaTiO3 (BT) ceramic with general formula Ba1-xBi2x/3TiO3, synthesized by conventional solid-state reaction route. The recorded room temperature XRD spectra show a tetragonal symmetry and the tetragonality reduces with Bi-doped derivatives. The temperature-dependent dielectric behavior of the compositions is studied and modification in the paraelectric-ferroelectric (PE-FE) phase transition is observed. The dielectric diffusivity increases with substitution of Bi3+ ion on A-site of BaTiO3 because of modified polar structure. The temperature coefficient of dielectric constant has been calculated and obtained values suggest that the composition x = 0.01 and 0.025 are suitable for X5R (− 15% ≤ \(\left( {\varepsilon - \in_{{25^{0} {\text{C}}}} } \right)/ \in_{{25^{0} {\text{C}}}}\) ≤ 15%, temperature range from − 55 to 85 °C) multi-layer ceramic capacitor (MLCC) application. A relaxor behavior has been observed for x = 0.1 and the Vogel-Fulcher fitting of the composition was carried out. The ferroelectric behavior illustrates that the coercive field and the remnant polarization increase up to x = 0.05 and decrease for higher doping. The energy storage efficiency for all the compositions has been calculated and the highest efficiency was obtained for x = 0.1. The optical property of all the synthesized samples has been studied using UV–Visible spectroscopy.

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Authors and Affiliations

  1. Department of Physics, Centurion University of Technology & Management, Jatni, Odisha, 752050, India

    A. K. Mahapatra & S. Sarangi

  2. Department of Physics, C.V. Raman Global University, Bhubaneswar, Odisha, 752054, India

    T. Badapanda

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  1. A. K. Mahapatra
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  2. T. Badapanda
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  3. S. Sarangi
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Mahapatra, A.K., Badapanda, T. & Sarangi, S. Compositional induced structural, dielectric, ferroelectric and optical study of Bismuth modified Barium Titanate ceramic. Appl. Phys. A 127, 593 (2021). https://doi.org/10.1007/s00339-021-04747-8

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