Skip to main content
Log in

A Reconsideration of Ştefania Mărăcineanu’s Measurements of Polonium-210’s Half-Life: Understanding Her Claim to the Discovery of Artificial Radioactivity

  • Published:
Physics in Perspective Aims and scope Submit manuscript

Abstract

I re-examine the raw data of the measurements of the half-life of 210Po from the Romanian physicist Ştefania Mărăcineanu’s doctoral thesis, performed at the Institut du Radium, 1921–1923, under the supervision of Marie Curie. The half-life values reported in the thesis show relatively large divergences and a possible dependence on the (metallic) support on which the Po source was deposited. These findings influenced Mărăcineanu’s subsequent independent research, and later compelled her to claim priority for the discovery of artificial radioactivity. The present analysis of these data, performed with the least-squares method, certifies the outstanding accuracy of the experimental measurements by providing values with good agreement between the different series of measurements and an average value that is close to the currently adopted half-life value of this isotope. On the other hand, this analysis changes our perspective by showing that the rudimentary procedure Mărăcineanu used to processing the data introduced errors in her reported values, which favored a poor interpretation of the results.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Fig. 1
Fig. 2

Source: Ştefania Mărăcineanu, Thèses présentées a la Faculté de Sciences de l’Université de Paris pour obtenir le grade de docteur ès sciences physiques (Paris: Les Presses Universitaires de France, 1924), 23

Fig. 3

Source: ENSDF – Evalated Nuclear Structure Data Files

Fig. 4

Source: Ştefania Mărăcineanu, Thèses présentées a la Faculté de Sciences de l’Université de Paris pour obtenir le grade de docteur ès sciences physiques (Paris: Les Presses Universitaires de France, 1924), 34

Fig. 5

Source: Ştefania Mărăcineanu, Thèses présentées a la Faculté de Sciences de l’Université de Paris pour obtenir le grade de docteur ès sciences physiques (Paris: Les Presses Universitaires de France, 1924), 32

Fig. 6

Similar content being viewed by others

References

  1. Ştefania Mărăcineanu, Thèses présentées a la Faculté de Sciences de l’Université de Paris pour obtenir le grade de docteur ès sciences physiques (Paris: Les Presses Universitaires de France, 1924).

  2. Ştefania Mărăcineanu, “Recherches sur le constante du polonium,” Comptes Rendus de l’Académie de Sciences 176 (1923), 1879–81; “Sur une méthode de mesure pour un fort rayonnement,” Comptes Rendus de l’Académie de Sciences 177 (1923), 682–85; “Recherches sur la penetration des substances radioactives dans les métaux,” Comptes Rendus de l’Académie de Sciences 177 (1923), 1215–17.

  3. Marco Fontani, Mary Virginia Orna, Mariagrazia Costa, and Sabine Vater, “Science is Not a Totally Transparent Structure: Ştefania Mărăcineanu and the Presumed Discovery of Artificial Radioactivity,” Substancia 1, no. 1 (2017) 77–96; Miruna Popescu, Marelene F. Rayner-Canham, and Geoffrey Rayner-Canham, “Stefania Maracineanu - Ignored Romanian Scientist,” in A Devotion to Their Science: Pioneer Women in Radioactivity, ed. Rayner-Canham and G.W. Rayner-Canham, 87–91 (Montreal: McGill-Queens University Press, 1977); Natalie Pigeard-Micault, “Stefania Maracineanu (1882–1944),” in Les femmes du laboratoire de Marie Curie, 164–72 (Paris: Glyphe, 2013).

  4. “The Nobel Prize in Chemistry 1935,” NobelPrize.org, accessed April 24, 2020, https://www.nobelprize.org/prizes/chemistry/1935/summary/.

  5. See the examples quoted in Fontani et al., “Science Is Not” (ref. 3).

  6. Mărăcineanu, Thèses (ref. 1).

  7. Mărăcineanu, Thèses (ref. 1).

  8. Mărăcineanu, Thèses (ref. 1), 59. All translations by the author unless otherwise stated.

  9. Mărăcineanu, “Recherches sur le constante”; “Sur une méthode”; “Recherches sur la penetration” (ref. 2).

  10. Ştefania Mărăcineanu, Records of the Romanian Academy of Sciences meeting, accessed on March 23, 2020, http://www.mnt-leonida.ro/09Noutati/090043Noutati2013.10.17/StMaracineanu2013AR.pdf (in Romanian).

  11. “Gespräch mit Irene Curie. Die tochter der radiumentdeckerin im Wien,” Neues Wiener Journal, June 5, 1934.

  12. Thanks to Prof. D.-P. Şerban for supplying a copy of this article and its translation.

  13. Ştefania Mărăcineanu, letter to Marie Curie, September 4, 1924, Museé Curie archives, Letter AIR LC.MC / Pièce 1075.

  14. Ştefania Mărăcineanu, letter to Marie Curie, October 26, 1924, Museé Curie archives, Letter AIR LC.MC / Pièce 1098.

  15. Stephanie Mărăcineanu, “Recherches sur l’effet du soleil au point de vue radioactive. Rayonnement émis par le plomb – effet des radiations solaires et de champs électriques et magnetiques,” Bulletin de la Section Scientifique de l’Académie Roumaine 11 (1925), 51–61.

    Google Scholar 

  16. Ştefania Mărăcineanu, letter to Marie Curie, November 5, 1924, Museé Curie archives, Letter AIR LC.MC / Pièce 1103.

  17. Ştefania Mărăcineanu, letter to Marie Curie, November 14, 1924, Museé Curie archives, Letter AIR LC.MC / Pièce 1105.

  18. Mărăcineanu, “Recherches sur l’effet du soleil” (ref. 15), 52.

  19. Mărăcineanu, Records of the Romanian Academy (ref. 10).

  20. More detailed discussion can be found in: Fontani et al., “Science Is Not” (ref. 3); Popescu et al., “Stefania Maracineanu” (ref. 3); and Pigeard-Micault, “Stefania Maracineanu (1882–1944)” (ref. 3).

  21. Ştefania Mărăcineanu, “Actions spéciales du Soleil sur la radioactivité du plomb et de l’uranium,” Comptes Rendus de l’Académie de Sciences 181 (1925), 774–76.

    Google Scholar 

  22. Mărăcineanu, Thèses (ref. 1), 53–57.

  23. Ştefania Mărăcineanu, “Effet special du polonium, du rayonnement solaire et de la haute tension sur le plomb,” Comptes Rendus de l’Académie de Sciences 184 (1927), 122–24.

    Google Scholar 

  24. Ştefania Mărăcineanu, “Sur les phénomènes semblables à ceux des corps radioactifs, présentés par les métaux,” Comptes Rendus de l’Académie de Sciences 186 (1928) 746–78.

    Google Scholar 

  25. For a detailed account, see Fontani et al., “Science Is Not” (ref. 3).

  26. Fontani et al., “Science Is Not” (ref. 3); Popescu et al., “Stefania Maracineanu” (ref. 3); and Pigeard-Micault, “Stefania Maracineanu (1882–1944)” (ref. 3).

  27. ENSDF (Evaluated Nuclear Structure Data File), accessed April 24, 2020, https://www.nndc.bnl.gov/ensdf/.

  28. Shaul Katzir, “The Discovery of the Piezoelectric Effect,” Archive for History of Exact Sciences 57, no. 1 (2003), 61–91.

    Article  MathSciNet  Google Scholar 

  29. Mărăcineanu, Thèses (ref. 1).

  30. Mărăcineanu, “Recherches sur le constante”; “Sur une méthode”; “Recherches sur la penetration” (ref. 2).

  31. “Least Squares,” Wikipedia, accessed March 20, 2020, https://en.wikipedia.org/wiki/Least_squares.

  32. ENSDF (ref. 27).

  33. Frédéric Joliot and Irène Curie, “Artificial Production of a New Kind of Radio-Element,” Nature 133 (1934), 201–2; Frédéric Joliot, “Chemical Evidence of the Transmutation of Elements,” Nobel Lecture, December 12, 1935, NobelPrize.org, accessed April 25, 1935, https://www.nobelprize.org/uploads/2018/06/joliot-fred-lecture.pdf.

  34. Mărăcineanu, “Sur les phénomènes” (ref. 24).

  35. Fontani et al., “Science Is Not” (ref. 3); Popescu et al., “Stefania Maracineanu” (ref. 3).

  36. Fontani et al., “Science Is Not” (ref. 3), 89.

  37. Fontani et al., “Science Is Not” (ref. 3).

  38. Elisabetg Rona and Ewald A. W. Schmidt, “Untersuchungen über das Eindringen des Poloniums in Metalle,” Sitzungsberichte der Akademie der Wissenschaften mathematisch-naturwissenschaftliche Klasse 136, no. 2a (1927), 65–73.

Download references

Acknowledgments

I would like to thank Mme. Natalie Pigeard for allowing my access to Ştefania Mărăcineanu’s letters from the Museé Curie archives.

Author information

Authors and Affiliations

Authors

Corresponding author

Correspondence to Dorel Bucurescu.

Additional information

Publisher's Note

Springer Nature remains neutral with regard to jurisdictional claims in published maps and institutional affiliations.

Dorel Bucurescu is senior researcher at the Horia Hulubei National Institute for Physics and Nuclear Engineering, and the Advanced Studies in Physics Center of the Romanian Academy, in Bucharest, Romania; his main field of research is nuclear spectroscopy.

Rights and permissions

Reprints and permissions

About this article

Check for updates. Verify currency and authenticity via CrossMark

Cite this article

Bucurescu, D. A Reconsideration of Ştefania Mărăcineanu’s Measurements of Polonium-210’s Half-Life: Understanding Her Claim to the Discovery of Artificial Radioactivity. Phys. Perspect. 22, 162–181 (2020). https://doi.org/10.1007/s00016-020-00259-9

Download citation

  • Published:

  • Issue Date:

  • DOI: https://doi.org/10.1007/s00016-020-00259-9

Keywords

Navigation