Abstract
The atmospheric concentration of 210Pb was determined for two years at six stations in the western North Pacific region. The following results were obtained and discussed by comparing them with those of Al. The atmospheric concentration of 210Pb varied widely from week to week, but the degree of variation was about a half that of Al. Contrary to Al, the year-to-year variation of 210Pb was not pronounced and its seasonal variation was well expressed by a sine curve. The 210Pb concentration did not show a marked latitudinal variation and its base-line concentration was high in the surface air over the North Pacific. These suggest that atmospheric 210Pb has a longer residence time, due to its transportation through higher altitudes and deposits much more evenly onto the Earth's surface and the ocean, as compared with Al in mineral dust which is larger in size in the source region.
Similar content being viewed by others
References
Burton, W. M. and Stewart, N. G., 1960, Use of long-lived natural radioactivity as an atmospheric tracer, Nature 186, 584–589.
Gavini, M. B., Beck, J. N., and Kuroda, P. K., 1974, Mean residence times of the long-lived radon daughters in the atmosphere, J. Geophys. Res. 79, 4447–4452.
Graustein, W. C. and Turekian, K. K., 1985, 210Pb traces the transport and deposition of continental aerosols to the mid-Pacific, Paper presented at IAMAP/IAPSO Joint Assembly, Honolulu, Hawaii, 5–16 August 1985.
Graustein, W. C. and Turekian, K. K., 1986, 210Pb and 137Cs in air and soils measure the rate and vertical profile of aerosol scavenging, J. Geophys. Res. 91, 14355–14366.
Kurata, T., 1986, Use of 210Pb, 210Bi and 210Po in the study of atmospheric transport of continental substances to the Ocean, Thesis for Doctor of Fisheries Sciences submitted to Hokkaido University.
Moore, H. E., Poet, S. E., and Martell, E. A., 1973, 222Rn, 210Pb, 210Bi and 210Po profiles and aerosol residence times versus altitude, J. Geophys. Res. 78, 7065–7075.
Poet, S.E., Moore, H. E., and Martell, E. A., 1972, Lead 210, bismuth 210 and polonium 210 in the atmosphere: a ccurate ratio measurement and application to aerosol residence time determination, J. Geophys. Res. 77, 6515–6527.
Prospero, J. M., Savoie, D. L., Nees, R. T., Duce, R. A. and Merrill, J. T., 1985, Particulate sulfate and nitrate in the boundary layer over the North Pacific Ocean, J. Geophys. Res. 90, 10586–10596.
Suzuki, T. and Tsunogai, S., 1988, Origin of calcium in aerosols over the western North Pacific, J. Atmos. Chem. 6, 363–374.
Turekian, K. K. and Cochran, J. K., 1981, 210Pb in surface air at Enewetak and the Asian dust flux to the Pacific, Nature 292, 522–524, Corrigenda, Nature 294, 670.
Turekian, K. K., Nozaki, Y., and Benninger, L. K., 1977, Geochemistry of atmospheric radon and radon products, Ann. Rev. Earth Planet. Sci. 5, 227–255.
Tsunogai, S., 1971, Oxidation rate of sulfite in water and its bearing on the origin of sulfate in meteoric precipitation, Geochem. J. 5, 57–67.
Tsunogai, S., 1979, Pb-210 and atmospheric residence times, Preprints of papers presented at the 177th National Meeting, Honolulu, Hawaii, 1–6 April 1979, 19, 389–392.
Tsunogai, S. and Fukuda, K., 1974, Pb-210, Bi-210 and Po-210 in meteoric Precipitation and the residence time of tropospheric aerosol, Geochem. J. 8, 141–152.
Tsunogai, S., Suzuki, T., Kurata, T., and Uematsu, M., 1985, Seasonal and areal variation of continental aerosol in the surface air over the western North Pacific region, J. Oceanogr. Soc. Japan 41, 427–434.
Uematsu, M., Duce, R. A., Prospero, J. M., Chen, L., Merrill, T., and McDonald, R. L., 1983, Transport of mineral aerosol from Asia over the North Pacific Ocean, J. Geophys. Res. 88, 5343–5352.
Author information
Authors and Affiliations
Rights and permissions
About this article
Cite this article
Tsunogai, S., Kurata, T., Suzuki, T. et al. Seasonal variation of atmospheric 210Pb and Al in the western North Pacific region. J Atmos Chem 7, 389–407 (1988). https://doi.org/10.1007/BF00058712
Received:
Revised:
Issue Date:
DOI: https://doi.org/10.1007/BF00058712