Abstract
Carbon dioxide dissociation using dielectric barrier discharge has been experimentally investigated. The electrical discharge was stimulated using high voltage pulses of nanosecond duration, with a repetition rate in the range of 100–1000 Hz. The reactor consisted of two stainless steel plane circular electrodes covered with either fused silica glasses or polytetrafluoroethylene (PTFE) films. Experiments were carried in pure CO2, and the concentration of carbon monoxide and ozone in the effluent gas was determined using UV/VIS and FTIR spectrophotometry. The results have shown that using silica as dielectric layers results in a higher generation efficiency for both CO and O3.
Access this chapter
Tax calculation will be finalised at checkout
Purchases are for personal use only
References
R. Snoeckx, A. Bogaerts, Plasma technology – a novel solution for CO2 conversion? Chem. Soc. Rev. 46, 5805–5863 (2017)
B. Ashford, Tu, X, Non-thermal plasma technology for the conversion of CO2. Curr. Opin. Green Sustain. Chem. 3, 45–49 (2017)
H. Kim, Nonthermal plasma processing for air-pollution control: a historical review, current issues, and future prospects. Plasma Process. Polym. 1, 91–110 (2004)
G.J. van Rooij, D.C. van den Bekerom, N. den Harder, T. Minea, G. Berden, W.A. Bongers, R. Engeln, M.F. Graswinckel, E. Zoethout, M.C. van de Sanden, Taming microwave plasma to beat thermodynamics in CO2 dissociation. Faraday Discuss. 183, 233–248 (2015)
R. Aerts, W. Somers, A. Bogaerts, Carbon dioxide splitting in a dielectric barrier discharge plasma: a combined experimental and computational study. ChemSusChem 8(4), 702–716 (2015)
M.S. Moss, K. Yanallah, R.W.K. Allen, F. Pontiga, An investigation of CO splitting using nanosecond pulsed corona discharge: effect of argon addition on CO conversion and energy efficiency. Plasma Sources Sci. Technol. 26(3), 035009 (2017)
A. Ozkan, T. Dufour, A. Bogaerts, F. Reniers, How do the barrier thickness and dielectric material influence the filamentary mode and CO conversion in a flowing DBD? Plasma Sources Sci. Technol. 25(4), 045016 (2016)
A. Fridman, Plasma Chemistry (Cambridge University Press, New York, 2008)
Acknowledgements
This research has been funded by the following organizations: Ministerio de Ciencia, Innovación y Universidades, Agencia Estatal de Investigación and Fondo Europeo de Desarrollo Regional, under contract no. PGC2018-099217-B-I00.
Author information
Authors and Affiliations
Corresponding author
Editor information
Editors and Affiliations
Rights and permissions
Copyright information
© 2020 Springer Nature Singapore Pte Ltd.
About this paper
Cite this paper
Pontiga, F., Guemou, M., Moreno, H., Fernández-Rueda, A., Yanallah, K. (2020). Carbon Dioxide Dissociation Using Pulsed DBD with Different Kinds of Dielectric Barriers. In: Belasri, A., Beldjilali, S. (eds) ICREEC 2019. Springer Proceedings in Energy. Springer, Singapore. https://doi.org/10.1007/978-981-15-5444-5_54
Download citation
DOI: https://doi.org/10.1007/978-981-15-5444-5_54
Published:
Publisher Name: Springer, Singapore
Print ISBN: 978-981-15-5443-8
Online ISBN: 978-981-15-5444-5
eBook Packages: EnergyEnergy (R0)