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Redox Chemistry of Sulfur, Selenium and Tellurium Compounds

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Selenium and Tellurium Chemistry

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Abstract

The oxidation of organochalcogen compounds to their corresponding radical cations and dications is described. The importance of through space and ‘secondary’ interactions in influencing this oxidation chemistry is illustrated in a number of cases.

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Notes

  1. 1.

    These model studies are challenging in their own right but further complicated by β-amyloid polymorphism [136].

  2. 2.

    Interestingly this model has been supplanted by one in which Met-35 is directed away from the hydrophobic interior of the peptide (containing the side-chain of Phe-19) toward the exterior where it is close to a second Met residue of another peptide in the oligomer. If oxidation of Met-35 is important in the pathogenesis of Alzheimer’s disease, this suggests the possibility of interaction between the two methionine sulfur atoms. As mentioned above, 1, 5-dithiocane 8, X = Y = S reduces Cu(II).

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  1. Department of Chemistry and Biochemistry, The University of Arizona, Tucson, AZ, 85721, USA

    Richard S. Glass

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  1. , School of Chemistry, University of St Andrews, UK, North Haugh, St. Andrews, KY16 9ST, United Kingdom

    J. Derek Woollins

  2. , Dept. of Chemistry, University of Oulu, PO Box 3000, Oulu, 90014, Finland

    Risto Laitinen

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Glass, R.S. (2011). Redox Chemistry of Sulfur, Selenium and Tellurium Compounds. In: Woollins, J., Laitinen, R. (eds) Selenium and Tellurium Chemistry. Springer, Berlin, Heidelberg. https://doi.org/10.1007/978-3-642-20699-3_3

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