Abstract
Using pump-probe spectroscopy, we investigate exciton-polariton dynamics in a strongly-coupled organic microcavity. We observe Rabi oscillations, decay of polaritons and the signature of the upper-branch cavity polaritons scattering to the exciton reservoir with phonon emission.
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References
D.G. Lidzey, D.D.C. Bradley, M.S. Skolnick, T. Virgili, S. Walker and D.M. Whittaker, “Strong exciton-photon coupling in an organic semiconductor microcavity” Nature 395, 53 (1998)
C. Manzoni, D. Polli and G. Cerullo “Two-color pump-probe system broadly tunable over the visible and the near infrared with sub-30 fs temporal resolution” Rev. Sci. Instrum. 77, 023103 (2006)
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Virgili, T., Ceccarelli, S., Polli, D., Lanzani, G., Cerullo, G., Lidzey, D.G. (2009). Temporal dynamics of polaritons in a stronglycoupled organic-semiconductor microcavity. In: Corkum, P., Silvestri, S., Nelson, K., Riedle, E., Schoenlein, R. (eds) Ultrafast Phenomena XVI. Springer Series in Chemical Physics, vol 92. Springer, Berlin, Heidelberg. https://doi.org/10.1007/978-3-540-95946-5_92
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DOI: https://doi.org/10.1007/978-3-540-95946-5_92
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Online ISBN: 978-3-540-95946-5
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