Skip to main content

Synergetic or Non-Linear Effects in PM10 and PM2.5 Scenario Calculations for 2015 in Belgium

  • Conference paper
Air Pollution Modeling and Its Application XIX

Abstract

We applied the extended version of the EUROS model to evaluate the impact of emission reductions on PM10 and PM2.5 concentrations in Flanders and Belgium for 2015. Individual sector contributions were assessed and the current and future changes in aerosol concentrations and compositions over Belgium and Europe were investigated. Contributions from anthropogenic sources in Flanders were found to be responsible for 34.3% of the annual averaged PM10 concentrations in Flanders in 2003. In 2015 this contribution is estimated to be 35.0%. For PM2.5 these contributions are 29.1% in 2003 and 27.8% in 2015 respectively. Results show that non-linear effects can not be neglected. Because of the non-linear processes that take place when secondary aerosols are formed, a small reduction in a gaseous compound (e.g. SO2) does not necessarily lead to the same amount of reduction of the secondary compound (e.g. sulphate). Another “non-linear” aspect is the formation of aerosols by contributions from two compounds that are delivered by two individual sectors. The synergetic effect of these “non-linear” contributions was found to be an additional 2.1% for PM10 and 3.7% for PM2.5, representing an increase of 6–13%, which is not negligible and might become relevant in abatement policies.

This is a preview of subscription content, log in via an institution to check access.

Access this chapter

Chapter
USD 29.95
Price excludes VAT (USA)
  • Available as PDF
  • Read on any device
  • Instant download
  • Own it forever
eBook
USD 84.99
Price excludes VAT (USA)
  • Available as PDF
  • Read on any device
  • Instant download
  • Own it forever
Softcover Book
USD 109.99
Price excludes VAT (USA)
  • Compact, lightweight edition
  • Dispatched in 3 to 5 business days
  • Free shipping worldwide - see info
Hardcover Book
USD 109.99
Price excludes VAT (USA)
  • Durable hardcover edition
  • Dispatched in 3 to 5 business days
  • Free shipping worldwide - see info

Tax calculation will be finalised at checkout

Purchases are for personal use only

Institutional subscriptions

Preview

Unable to display preview. Download preview PDF.

Unable to display preview. Download preview PDF.

References

  • Deutsch F, Janssen L, Vankerkom J, Lefebre F, Mensink C, Fierens F, Dumont G, Roekens E (2008) Modelling changes of aerosol compositions over Belgium and Europe, Int. J. Environ. Pollut. 32, 162-173.

    Article  CAS  Google Scholar 

  • Dockery DW, 3rd Pope CA, Xiping X, Spengler JD, Ware JH, Fay MA, Ferries BG Jr, Speizer FE (1993) An association between air pollution and mortality in six US cities. N. Engl. J. Med., 329(24), 1753-1759.

    Article  CAS  Google Scholar 

  • Griffin RJ, Dabdub D, Seinfeld JH (2002) Secondary organic aerosol 1. Atmospheric chemical mechanism for production of molecular constituents, J. Geophys. Res. 107(D17), 4332, doi:10.1029/2001JD000541.

    Article  Google Scholar 

  • Meng Z, Dabdub D, Seinfeld JH (1998) Size-resolved and chemically resolved model of atmospheric aerosol dynamics, J. Geophys. Res. 103, 3419-3435.

    Article  CAS  Google Scholar 

  • Nenes A, Pandis SN, Pilinis C (1998) ISORROPIA: a new thermodynamic equili-brium model for multiphase multicomponent inorganic aerosols, Aquatic Geo-chemistry 4, 123-152.

    Article  CAS  Google Scholar 

  • Pope CA 3rd, Burnett RT, Thun MJ (2002) Lung cancer, cardiopulmonary mortality and long-term exposure to fine particulate air pollution. JAMA, 287, 1132-1141.

    Article  CAS  Google Scholar 

  • Pun BK, Griffin RJ, Seigneur C, Seinfeld JH (2002) Secondary organic aerosol 2. Thermodynamic model for gas/particle partitioning of molecular constituents, J. Geophys. Res. 107(D17), 4333, AAC 4-1-4-15.

    Article  Google Scholar 

  • Vestreng V et al. (2005) Inventory Review 2005. Emission data reported to LRTAP and NEC Directive, initial review of HMs and POPs, EMEP/EEA Joint Review Report, EMEP/MSC-W Note 1, July 2005.

    Google Scholar 

  • VMM (2004) Lozingen in de lucht 1990-2003, Vlaamse Milieumaatschappij, Aalst, Belgium, 185 pp. +Appendix (in Dutch).

    Google Scholar 

  • Zhang Y, Pun B, Vijayaraghavan K, Wu S-Y, Seigneur C, Pandis SN, Jacobson MZ, Nenes A, Seinfeld JH (2004) Development and application of the Model of Aerosol Dynamics, Reaction, Ionization, and Dissolution (MADRID), J. Geophys. Res. 109, D01202, doi:10.1029/2003JD003501.

    Article  Google Scholar 

Download references

Authors

Editor information

Editors and Affiliations

Rights and permissions

Reprints and permissions

Copyright information

© 2008 Springer Science + Business Media B.V

About this paper

Cite this paper

Mensink, C., Deutsch, F., Vankerkom, J., Janssen, L. (2008). Synergetic or Non-Linear Effects in PM10 and PM2.5 Scenario Calculations for 2015 in Belgium. In: Borrego, C., Miranda, A.I. (eds) Air Pollution Modeling and Its Application XIX. NATO Science for Peace and Security Series Series C: Environmental Security. Springer, Dordrecht. https://doi.org/10.1007/978-1-4020-8453-9_28

Download citation

Publish with us

Policies and ethics