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Laser-Induced Ultrafast Demagnetization: Femtomagnetism, a New Frontier?

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Spin Dynamics in Confined Magnetic Structures I

Part of the book series: Topics in Applied Physics ((TAP,volume 83))

Abstract

The conventional demagnetization process (spin precession, magnetic domain motion and rotation) is governed mainly by spin—lattice, magnetic dipole and Zeeman, and spin-spin interactions. It occurs on a timescale of nanoseconds. Technologically, much faster magnetization changes are always in great demand to improve data processing speed. Unfortunately, the present speed of magnetic devices is already at the limit of the conventional mechanism with little room left. Fortunately and unprecedentedly, recent experimental investigations have evidenced much faster magnetization dynamics which occurs on a femtosecond time scale: femtomagnetism. This novel spin dynamics has not been well-understood until now. This article reviews the current status of ultrafast spin dynamics and presents a perspective for future experimental and theoretical investigations.

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References

  1. M. H. Kryder: Magneto-optic recording technology, J. Appl. Phys. 57, 3913 (1985)

    Article  ADS  Google Scholar 

  2. A. Vaterlaus, T. Beutler, F. Meier: Spin-lattice relaxation time of ferromagnetic gadolinium determined with time-resolved spin-polarized photoemission, Phys. Rev. Lett. 67, 3314 (1991)

    Article  ADS  Google Scholar 

  3. L. Landau, E. Lifshitz: On the theory of the dispersion of magnetic permeability in ferromagnetic bodies, Physik Z. Sowjetunion 8, 153 (1935)

    MATH  Google Scholar 

  4. W. Hübner, G. P. Zhang: Ultrafast spin dynamics in nickel, Phys. Rev. B 58, R5920 (1998)

    Article  ADS  Google Scholar 

  5. G. D. Mahan: Many-Body Physics, 2nd ed. (Plenum, New York 1990)

    Google Scholar 

  6. E. Beaurepaire, J.-C. Merle, A. Daunois, J. Y. Bigot: Ultrafast spin dynamics in ferromagnetic nickel, Phys. Rev. Lett. 76, 4250 (1996)

    Article  ADS  Google Scholar 

  7. J. Hohlfeld, E. Matthias, R. Knorren, K. H. Bennemann: Nonequilibrium magnetization dynamics of nickel, Phys. Rev. Lett. 78, 4861 (1997); ibid. 79, 960 (1997) (erratum)

    Article  ADS  Google Scholar 

  8. A. Scholl, L. Baumgarten, W. Eberhardt: Ultrafast spin dynamics of ferromagnetic thin films observed by fs spin-resolved two-photon photoemission, Phys. Rev. Lett. 79, 5146 (1997)

    Article  ADS  Google Scholar 

  9. M. Aeschlimann, M. Bauer, S. Pawlik, W. Weber, R. Burgermeister, D. Oberli, H. C. Siegmann: Ultrafast spin-dependent electron dynamics in fcc Co, Phys. Rev. Lett. 79, 5158 (1997)

    Article  ADS  Google Scholar 

  10. E. Beaurepaire, M. Maret, V. Halte, J.-C. Merle, A. Daunois, J. Y. Bigot: Spin dynamics in CoPt3 alloy films: A magnetic phase transition in the femtosecond timescale, Phys. Rev. B 58, 12134 (1998)

    Article  ADS  Google Scholar 

  11. G. P. Zhang, W. Hübner: Femtosecond electron and spin dynamics probed by nonlinear optics, Appl. Phys. B 68, 495 (1999); G. P. Zhang, W. Hübner: Femtosecond spin dynamics in the time domain, J. Appl. Phys. 85, 5657 (1999)

    Article  ADS  Google Scholar 

  12. W. Hübner, G. P. Zhang: Femtosecond spin dynamics probed by linear and nonlinear magneto-optics, J. Magn. Magn. Mater. 189, 101 (1998)

    Article  ADS  Google Scholar 

  13. G. Ju, A. Vertikov, A. V. Nurmikko, C. Canady, G. Xiao, R. F. C. Farrow, A. Cebollada: Ultrafast nonequilibrium spin dynamics in a ferromagnetic thin film, Phys. Rev. B 57, R700 (1998)

    Article  ADS  Google Scholar 

  14. W. Heisenberg: Z. Phys. 49, 619 (1928)

    Article  ADS  Google Scholar 

  15. T. Holstein, H. Primakoff: Field dependence of the intrinsic domain magnetization of a ferromagnet, Phys. Rev. 58, 1098 (1940)

    Article  MATH  ADS  Google Scholar 

  16. J. Hubbard: Proc. R. Soc. London A 276, 238 (1963)

    Article  ADS  Google Scholar 

  17. P. Fulde: Electron Correlation in Molecules and Solids, 3rd ed. (Springer, Berlin, Heidelberg 1995)

    Google Scholar 

  18. J. Wahle, N. Blümer, J. Schling, K. Held, D. Vollhardt: Microscopic conditions favoring itinerant ferromagnetism, cond-mat/9711242

    Google Scholar 

  19. E. C. Stoner: Collective electron ferromagnetism, Proc. R. Soc. London A 165, 372 (1938); Collective electron ferromagnetism II. Energy and specific heat, ibid. A 169, 339 (1939)

    Article  ADS  Google Scholar 

  20. R. Orbach: Proc. R. Soc. London A 264, 458 (1961) and 264, 485 (1961)

    Article  ADS  Google Scholar 

  21. P. L. Scott, C. D. Jeffries: Spin-lattice relaxation in some rare-earth salts at helium temperatures, Phys. Rev. 127, 32 (1962)

    Article  ADS  Google Scholar 

  22. W. Hübner: Theory of nonlinear surface magneto-optics for ferromagnetic nickel: Effects of band structure and matrix elements, Phys. Rev. B 42, 11553 (1990); A. Lessard, T. H. Moos, W. Hübner: Magnetocrystalline anisotropy energy of transition-metal thin films: A nonperturbative theory, Phys. Rev. B 56, 2594 (1997); T. H. Moos, W. Hübner, K. H. Bennemann: Magnetocrystalline anisotropy of a transition metal monlayer: A non-perturbative theory, Solid State Commun. 98, 639 (1996)

    Article  ADS  Google Scholar 

  23. W. Hübner, L. M. Falicov: Theory of spin-polarized electron-capture spec-troscopy in ferromagnetic nickel, Phys. Rev. B 47, 8783 (1993); C. Moore: Atomic Energy Levels, Natl. Bur. Stand. (U.S.) (U.S. GPO, Washington, DC 1971)

    Article  ADS  Google Scholar 

  24. H. Takayama, K. Bohnen, P. Fulde: Magnetic surface anisotropy of transition metals, Phys. Rev. B 14, 2287 (1976)

    Article  ADS  Google Scholar 

  25. W. L. O’Brien, B. P. Tonner: Orbital and spin sum rules in X-ray magnetic circular dichroism, Phys. Rev. B 50, 12672 (1994)

    Article  ADS  Google Scholar 

  26. S. Hüfner, G. K. Wertheim, N. V. Smith, M. M. Traum: Solid State Commun. 11, 323 (1972); C. Guillot, Y. Ballu, J. Paigné, J. Lecante, K. P. Jain, P. Thiry, R. Pinchaux, Y. P’etroff, L. M. Falicov: Resonant photoemission in nickel metal, Phys. Rev. Lett. 39, 1632 (1977)

    Article  Google Scholar 

  27. N. I. Zheludev, P. J. Bennett, H. Loh, S. V. Popov, I. R. Shatwell, Y. P. Svirko, V. E. Gusev, V. F. Kamalov, E. V. Slobodchikov: Cubic optical nonlinearity of free electrons in bulk gold, Opt. Lett. 20, 1368 (1995)

    Article  ADS  Google Scholar 

  28. P. Kner, S. Bar-Ad, M. V. Marquezini, D. S. Chemla, W. Schäfer: Magnetically enhanced exciton-exciton correlations in semiconductors, Phys. Rev. Lett. 78, 1319 (1997)

    Article  ADS  Google Scholar 

  29. G. L. Eesley: Observation of nonequilibrium electron heating in copper, Phys. Rev. Lett. 51, 2140 (1983)

    Article  ADS  Google Scholar 

  30. H. E. Elsayed-Ali, T. B. Norris, M. A. Pessot, G. A. Mourou: Time-resolved observation of electron-phonon relaxation in copper, Phys. Rev. Lett. 58, 1212 (1987)

    Article  ADS  Google Scholar 

  31. R. W. Schoenlein, W. Z. Lin, J. G. Fujimoto, G. L. Eesley: Femtosecond studies of nonequilibrium electronic processes in metals, Phys. Rev. Lett. 58, 1680 (1987)

    Article  ADS  Google Scholar 

  32. S. D. Brorson, A. Kazeroonian, J. S. Moodera, D. W. Face, T. K. Cheng, E. P. Ippen, M. S. Dresselhaus, G. Dresselhaus: Femtosecond room-temperature measurement of the electron-phonon coupling constant gamma in metallic superconductors, Phys. Rev. Lett. 64, 2172 (1990)

    Article  ADS  Google Scholar 

  33. R. H. M. Groeneveld, R. Sprik, A. Lagendijk: Effect of a nonthermal electron distribution on the electron-phonon energy relaxation process in noble metals, Phys. Rev. B 45, 5079 (1992)

    Article  ADS  Google Scholar 

  34. W. S. Fann, R. Storz, H. W. K. Tom, J. Bokor: Direct measurement of nonequi-librium electron-energy distributions in subpicosecond laser-heated gold films, Phys. Rev. Lett. 68, 2834 (1992)

    Article  ADS  Google Scholar 

  35. T. Q. Qiu, C. L. Tien: Heat transfer mechanisms during short-pulse laser heating of metals, Int. J. Heat Mass Transfer 35, 719 (1992)

    Article  ADS  Google Scholar 

  36. C.-K. Sun, F. Vallée, L. H. Acioli, E. P. Ippen, J. G. Fujimoto: Femtosecond-tunable measurement of electron thermalization in gold, Phys. Rev. B 50, 15337 (1994)

    Article  ADS  Google Scholar 

  37. For a recent review on the electron dynamics in metals, see the whole issue of Chem. Phys. 251 (2000)

    Google Scholar 

  38. M. I. Kaganov, I. M. Lifshits, L. V. Tanatarov: Sov. Phys. JETP 4, 173 (1957)

    MATH  Google Scholar 

  39. S. I. Anisimov, B. L. Kapeliovich, T. L. Perel’man: Electron emission from metal surfaces exposed to ultrashort laser pulse, Sov. Phys. JETP 39, 375 (1974)

    ADS  Google Scholar 

  40. P. B. Allen: Theory of thermal relaxation of electrons in metals, Phys. Rev. Lett. 59, 1460 (1987)

    Article  ADS  Google Scholar 

  41. C. Suarez, W. E. Bron, T. Juhasz: Dynamics and transport of electronic carriers in thin gold films, Phys. Rev. Lett. 75, 4536 (1995)

    Article  ADS  Google Scholar 

  42. V. E. Gusev, O. B. Wright: Ultrafast nonequilibrium dynamics of electrons in metals, Phys. Rev. B 57, 2878 (1998)

    Article  ADS  Google Scholar 

  43. D. Pines, P. Nozières: The Theory of Quantum Liquids (Benjamin, New York 1966)

    Google Scholar 

  44. R. Rosei, D. W. Lynch: Thermomodulation spectra of Al, AU and Cu, Phys. Rev. B 5, 3883 (1972)

    Article  ADS  Google Scholar 

  45. N. W. Ashcroft, N. D. Mermin: Solid State Physics (Saunders College, Philadelphia 1976)

    Google Scholar 

  46. J.-Y. Bigot, E. Beaurepaire, A. Daunois, J.-C. Merle: in Ultrafast Phenomena X, Springer Ser. Chem. Phys. 62, P. F. Barbara, J. G. Fujimoto, W. H. Knox, W. Zinth (Eds.) (Springer, Berlin, Heidelberg 1996)

    Google Scholar 

  47. M. B. Agranat, S. I. Ashitkov, A. B. Granovskii, G. I. Rukman: Interaction of picosecond laser pulses with the electron, spin an phonon subsystems of nickel, Sov. Phys.-JETP 59, 804 (1984)

    Google Scholar 

  48. A. Y. Elezzabi, M. R. Freeman, M. Johnson: Direct measurement of the conduction electron spin-lattice relaxation time T1 in Gold, Phys. Rev. Lett. 77, 3220 (1996)

    Article  ADS  Google Scholar 

  49. W. Voigt: Magneto-und Electro-Optik, (Teubner, Leipzig 1908)

    Google Scholar 

  50. P. M. Oppeneer, T. Maurer, J. Sticht, J. Kübler: Ab initio calculated magneto-optical Kerr effect of ferromagnetic metals: Fe and Ni, Phys. Rev. B 45, 10924 (1992); P. M. Oppeneer, J. Sticht, T. Maurer, J. Kübler: Ab initio investigation of microscopic enhancement factors in tuning the magneto-optical Kerr effect, Z. Phys. B 88, 309 (1992)

    Article  ADS  Google Scholar 

  51. Q. Y. Jin, H. Regensburger, R. Vollmer, J. Kirschner: Periodic oscillations of the surface magnetization during the growth of Co films on Cu(001), Phys. Rev. Lett. 80, 4056 (1998)

    Article  ADS  Google Scholar 

  52. T. Rasing: Nonlinear magneto-optical probing of magnetic interfaces, Appl. Phys. B 68, 477 (1999)

    Article  ADS  Google Scholar 

  53. B. Koopmans, A. M. Janner, H. A. Wierenga, T. Rasing, G. A. Sawatzky, F. van der Woude: Separation of interface and bulk contributions in second-harmonic generation from magnetic and non-magnetic multilayers, Appl. Phys. A 60, 103 (1995)

    Article  ADS  Google Scholar 

  54. W. Hübner, K. H. Bennemann: Electronic theory for the nonlinear magneto-optical response of transition metals at surfaces and interfaces: Dependence of the Kerr rotation on the polarization and magnetic easy axis, Phys. Rev. B 52, 13411 (1995)

    Article  ADS  Google Scholar 

  55. V. V. Pavlov, G. Tessier, C. Malouin, P. Georges, A. Brun, D. Renard, P. Meyer, J. Ferré, P. Beauvillain: Observation of magneto-optical second-harmonic generation with surface plasmon excitation in ultrathin Au/Co/Au films, Appl. Phys. Lett. 75, 190 (1999)

    Article  ADS  Google Scholar 

  56. M. Maret, M.-C. Cadeville, R. Poinsot, A. Herr, E. Beaurepaire, C. Monier: Structural order related to the magnetic anisotropy in epitaxial (111) CoPt3 alloy films, J. Magn. Magn. Mater. 166, 45 (1997)

    Article  ADS  Google Scholar 

  57. U. Conrad, J. Güdde, V. Jahnke, E. Matthias: Ultrafast electron and magnetization dynamics of thin Ni and Co films on Cu(001) observed by time-resolved SHG, Appl. Phys. B 68, 511 (1999)

    Article  ADS  Google Scholar 

  58. J. Hohlfeld, J. Güdde, U. Conrad, O. Duhr, G. Korn, E. Matthias: Ultrafast magnetization dynamics of nickel, Appl. Phys. B 68, 505 (1999) J. Güdde, U. Conrad, V. Jähnke, J. Hohlfeld, E. Matthias: Magnetization dynamics of Ni and Co films on Cu(001) and of bulk nickel surfaces, Phys. Rev. B 59, R6608 (1999)

    Article  ADS  Google Scholar 

  59. B. Koopmans, M. van Kampen, J. T. Kohlhepp, W. J. M. de Jonge: Femtosecond spin dynamics of epitaxial Cu(111)/Ni/Cu wedges, J. Appl. Phys 87, 5070 (2000) B. Koopmans, M. van Kampen, J. T. Kohlhepp, W. J. M. de Jonge: Ultrafast magneto-optics in nickel: Magnetism or optics? Phys. Rev. Lett. 85, 844 (2000)

    Article  ADS  Google Scholar 

  60. J. Kessler: Polarized Electrons, 2nd ed. (Springer Verlag, Berlin 1985)

    Google Scholar 

  61. M. Campagna, D. T. Pierce, F. Meier, K. Sattler, H. C. Siegmann: Emission of Polarized Electrons in Solids in Advances in Electronics and Electron Physics, Vol. 41 (Academic, London 1976) p. 113

    Google Scholar 

  62. C. J. Lin, G. L. Gorman: Evaporated CoPt alloy films with strong perpendicular magnetic anisotropy, Appl. Phys. Lett. 61, 1600 (1992)

    Article  ADS  Google Scholar 

  63. L. Guidoni, E. Beaurepaire, J.-Y. Bigot: Magnetization dynamics in the femtosecond time scale in ferromagnetic metals, in Quantum Electronics Laser Science Conference, OSA Technical Digest Series (Opt. Soc. Am., Washington, DC 2000) p. 160

    Google Scholar 

  64. K. H. Bennemann: Ultrafast spin dynamics of magnetic metals in a nonequi-librium state, Rev. Mex. Fis. 44, 533 (1998)

    Google Scholar 

  65. J. S. Dodge, A. B. Schumacher, J.-Y. Bigot, D. S. Chemla, N. Ingle, M. R. Beasley: Time-resolved optical observation of spin-wave dynamics, Phys. Rev. Lett. 83, 4650 (1999)

    Article  ADS  Google Scholar 

  66. P. J. Bennett, V. Albanis, Yu. P. Svirko, N. I. Zheludev: Femtosecond cubic optical nonlinearity of thin nickel films, Opt. Lett. 24, 1373 (1999)

    Article  ADS  Google Scholar 

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Zhang, G., Hübner, W., Beaurepaire, E., Bigot, JY. (2002). Laser-Induced Ultrafast Demagnetization: Femtomagnetism, a New Frontier?. In: Hillebrands, B., Ounadjela, K. (eds) Spin Dynamics in Confined Magnetic Structures I. Topics in Applied Physics, vol 83. Springer, Berlin, Heidelberg. https://doi.org/10.1007/3-540-40907-6_8

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