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Source and seasonal variation in the major ion chemistry of two eastern Himalayan high altitude lakes, India

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Abstract

A chemical survey of two high-altitudes lakes, i.e., Tsokyo Tso and Sella, was conducted during pre-monsoon (May) and post-monsoon (November) 2011. Lake water is found to be pure with very low EC values even lesser than rainwater. This shows where lake water receives most of its contribution. A comprehensive and systematic study on the seasonal pattern of major ions (Cl, PO4 3−, HCO3 , NO3 , SO4 2−, Na+, K+, Ca2+, Mg2+, and SiO2) was carried out to understand the geochemical processes controlling water quality. There was marked seasonal variation observed for almost all ions. Factor analysis identifies geochemical controls, snow melting, and evaporative enrichment as main controlling factor. The partial pressure of CO2 (pCO2) value has increased in the post-monsoon probably due to higher atmospheric CO2 during winter. Overall, factor analysis identified processes like geochemical control, snowmelt water input, and evaporative enrichment in the pre-monsoon, atmospheric input and dilution of ions due to rainfall, microbial activities, and accumulation of weathered material lake system in the post-monsoon as governing processes switching among themselves in different seasons. HYSPILT back trajectory model was used to trace the source of long-range transport of pollutant. Results show for both the lakes that air arriving to the vicinity of the lake has an origin from the southeast direction during pre-monsoon and the mid-Gangetic plain during post-monsoon season, respectively. The results show that both the studied lakes have significant impacts of long-range transport of air pollutants rather than local interferences. Long-term monitoring of the fluctuation in key parameters can further verify the findings of this study.

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Acknowledgments

The authors gratefully acknowledge the NOAA Air Resources Laboratory (ARL) for the provision of the HYSPLIT transport and dispersion model and/or READY website (http://www.ready.noaa.gov) used in this publication. Authors also acknowledge the seed money grant from the Tezpur University partly used for this research.

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Correspondence to Manish Kumar.

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Deka, J.P., Tayeng, G., Singh, S. et al. Source and seasonal variation in the major ion chemistry of two eastern Himalayan high altitude lakes, India. Arab J Geosci 8, 10597–10610 (2015). https://doi.org/10.1007/s12517-015-1964-7

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  • DOI: https://doi.org/10.1007/s12517-015-1964-7

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