• Open Access

Ferromagnetism and Conductivity in Atomically Thin SrRuO3

H. Boschker, T. Harada, T. Asaba, R. Ashoori, A. V. Boris, H. Hilgenkamp, C. R. Hughes, M. E. Holtz, L. Li, D. A. Muller, H. Nair, P. Reith, X. Renshaw Wang, D. G. Schlom, A. Soukiassian, and J. Mannhart
Phys. Rev. X 9, 011027 – Published 8 February 2019
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Abstract

Atomically thin ferromagnetic and conducting electron systems are highly desired for spintronics, because they can be controlled with both magnetic and electric fields. We present (SrRuO3)1(SrTiO3)5 superlattices and single-unit-cell-thick SrRuO3 samples that are capped with SrTiO3. We achieve samples of exceptional quality. In these samples, the electron systems comprise only a single RuO2 plane. We observe conductivity down to 50 mK, a ferromagnetic state with a Curie temperature of 25 K, and signals of magnetism persisting up to approximately 100 K.

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  • Received 25 July 2018
  • Revised 22 October 2018

DOI:https://doi.org/10.1103/PhysRevX.9.011027

Published by the American Physical Society under the terms of the Creative Commons Attribution 3.0 License. Further distribution of this work must maintain attribution to the author(s) and the published article’s title, journal citation, and DOI.

Published by the American Physical Society

Physics Subject Headings (PhySH)

Condensed Matter, Materials & Applied Physics

Authors & Affiliations

H. Boschker1, T. Harada1, T. Asaba2, R. Ashoori3, A. V. Boris1, H. Hilgenkamp4, C. R. Hughes1,5, M. E. Holtz6, L. Li2,3, D. A. Muller6,7, H. Nair8, P. Reith4, X. Renshaw Wang4,*, D. G. Schlom7,8, A. Soukiassian8, and J. Mannhart1

  • 1Max Planck Institute for Solid State Research, 70569 Stuttgart, Germany
  • 2Department of Physics, University of Michigan, Ann Arbor, Michigan 48109, USA
  • 3Department of Physics, Massachusetts Institute of Technology, Cambridge, Massachusetts 02139, USA
  • 4MESA+ Institute for Nanotechnology, University of Twente, Enschede, Netherlands
  • 5Experimental Physics VI, Center for Electronic Correlations and Magnetism, Augsburg University, 86135 Augsburg, Germany
  • 6School of Applied and Engineering Physics, Cornell University, Ithaca, New York 14853, USA
  • 7Kavli Institute at Cornell for Nanoscale Science, Ithaca, New York 14853, USA
  • 8Department of Materials Science and Engineering, Cornell University, Ithaca, New York 14853, USA

  • *Present address: School of Physical and Mathematical Sciences and School of Electrical and Electronic Engineering, Nanyang Technological University, Singapore 637371, Singapore.

Popular Summary

Atomically thin materials that are both magnetic and conductive offer great promise for applications in spintronics, where information can be stored and transferred via the manipulation of electron spin. However, finding a material that meets all the requisite criteria is a challenge. Transition-metal oxides circumvent many of the problems encountered in other systems. One such material, SrRuO3, is already widely used in various applications, but previous research has suggested that it loses its magnetism when less than a few atoms thick. Our experiments show, however, that a single layer of SrRuO3 remains magnetic and conductive if it is embedded in a block of SrTiO3.

We discover that replacing a single TiO2 plane of SrTiO3 by a RuO2 plane causes this layer to be a conducting, 2D magnet. Over a temperature range of 2–300 K, the resistivity of the SrRuO3 layer remains well below that seen in previous studies. We also observe magnetic hysteresis at temperatures below 25 K and hints of magnetism up to 100 K. This is the first realization of a conducting electron system in a complex oxide heterostructure that is confined to a single atomic layer.

Such atomically thin magnetic conductors could help improve the understanding of 2D magnetism. Because they are expected to be tunable by electric fields, such systems could also find use in active spintronics devices.

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Vol. 9, Iss. 1 — January - March 2019

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