Biscale chaos in propagating fronts

Anatoly Malevanets, Agustí Careta, and Raymond Kapral
Phys. Rev. E 52, 4724 – Published 1 November 1995
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Abstract

The propagating chemical fronts found in cubic autocatalytic reaction-diffusion processes are studied. Simulations of the reaction-diffusion equation near to and far from the onset of the front instability are performed and the structure and dynamics of chemical fronts are studied. Qualitatively different front dynamics are observed in these two regimes. Close to onset the front dynamics can be characterized by a single length scale and described by the Kuramoto-Sivashinsky equation. Far from onset the front dynamics exhibit two characteristic lengths and cannot be modeled by this amplitude equation. An amplitude equation is proposed for this biscale chaos. The reduction of the cubic autocatalysis reaction-diffusion equation to the Kuramoto-Sivashinsky equation is explicitly carried out. The critical diffusion ratio δc, where the planar front loses its stability to transverse perturbations, is determined and found to be δc=2.300.

  • Received 25 May 1995

DOI:https://doi.org/10.1103/PhysRevE.52.4724

©1995 American Physical Society

Authors & Affiliations

Anatoly Malevanets, Agustí Careta, and Raymond Kapral

  • Chemical Physics Theory Group, Department of Chemistry, University of Toronto, Toronto, Canada M5S 1A1

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Issue

Vol. 52, Iss. 5 — November 1995

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