Nuclear excitation by electronic transition of U235

P. A. Chodash, J. T. Harke, E. B. Norman, S. C. Wilks, R. J. Casperson, S. E. Fisher, K. S. Holliday, J. R. Jeffries, and M. A. Wakeling
Phys. Rev. C 93, 034610 – Published 11 March 2016

Abstract

Background: Nuclear excitation by electronic transition (NEET) is a rare nuclear excitation that can occur in isotopes containing a low-lying nuclear excited state. Over the past 40 yr, several experiments have attempted to measure NEET of U235 and those experiments have yielded conflicting results.

Purpose: An experiment was performed to determine whether NEET of U235 occurs and to determine its excitation rate.

Method: A pulsed Nd:YAG laser operating at 1064 nm with a pulse energy of 790 mJ and a pulse width of 9 ns was used to generate a uranium plasma. The plasma was collected on a catcher plate and electrons from the catcher plate were accelerated and focused onto a microchannel plate detector. An observation of a decay with a 26-min half-life would suggest the creation of U235m and the possibility that NEET of U235 occurred.

Results: A 26-min decay consistent with the decay of U235m was not observed and there was no evidence that NEET occurred. An upper limit for the NEET rate of U235 was determined to be λNEET<1.8×104 s1, with a confidence level of 68.3%.

Conclusions: The upper limit determined from this experiment is consistent with most of the past measurements. Discrepancies between this experiment and past measurements can be explained by assuming that past experiments misinterpreted the data.

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  • Received 15 December 2015

DOI:https://doi.org/10.1103/PhysRevC.93.034610

©2016 American Physical Society

Physics Subject Headings (PhySH)

Nuclear Physics

Authors & Affiliations

P. A. Chodash1,*, J. T. Harke2, E. B. Norman1, S. C. Wilks3, R. J. Casperson2, S. E. Fisher4, K. S. Holliday5, J. R. Jeffries5, and M. A. Wakeling6

  • 1Department of Nuclear Engineering, University of California, Berkeley, California 94720, USA
  • 2Nuclear and Chemical Sciences Division, Lawrence Livermore National Laboratory, Livermore, California 94550, USA
  • 3Physics Division, Lawrence Livermore National Laboratory, Livermore, California 94550, USA
  • 4National Security Engineering Division, Lawrence Livermore National Laboratory, Livermore, California 94550, USA
  • 5Materials Science Division, Lawrence Livermore National Laboratory, Livermore, California 94550, USA
  • 6Air Force Institute of Technology, Wright-Patterson Air Force Base, Ohio 45433, USA

  • *Present address: Lawrence Livermore National Laboratory, Livermore, California 94550, USA.

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Issue

Vol. 93, Iss. 3 — March 2016

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