Magnetoexcitons and Faraday rotation in single-walled carbon nanotubes and graphene nanoribbons

Jonas Have and Thomas G. Pedersen
Phys. Rev. B 97, 115405 – Published 5 March 2018

Abstract

The magneto-optical response of single-walled carbon nanotubes (CNTs) and graphene nanoribbons (GNRs) is studied theoretically, including excitonic effects. Both diagonal and nondiagonal response functions are obtained and employed to compute Faraday rotation spectra. For single-walled CNTs in a parallel field, the results show field-dependent splitting of the exciton absorption peaks caused by brightening a dark exciton state. Similarly, for GNRs in a perpendicular magnetic field, we observe a field-dependent shift of the exciton peaks and the emergence of an absorption peak above the energy gap. Results show that excitonic effects play a significant role in the optical response of both materials, particularly for the off-diagonal tensor elements.

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  • Received 4 December 2017

DOI:https://doi.org/10.1103/PhysRevB.97.115405

©2018 American Physical Society

Physics Subject Headings (PhySH)

Condensed Matter, Materials & Applied Physics

Authors & Affiliations

Jonas Have1,2,* and Thomas G. Pedersen1,3

  • 1Department of Materials and Production, Aalborg University, DK-9220 Aalborg East, Denmark
  • 2Department of Mathematical Sciences, Aalborg University, DK-9220 Aalborg East, Denmark
  • 3Center for Nanostructured Graphene (CNG), DK-9220 Aalborg East, Denmark

  • *jh@nano.aau.dk

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Vol. 97, Iss. 11 — 15 March 2018

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