Dyadic Green's function formalism for photoinduced forces in tip-sample nanojunctions

Faezeh Tork Ladani and Eric Olaf Potma
Phys. Rev. B 95, 205440 – Published 31 May 2017

Abstract

A comprehensive theoretical analysis of photoinduced forces in an illuminated nanojunction, formed between an atomic force microscopy tip and a sample, is presented. The formalism is valid within the dipolar approximation and includes multiple scattering effects between the tip, sample, and a planar substrate through a dyadic Green's function approach. This physically intuitive description allows a detailed look at the quantitative contribution of multiple scattering effects to the measured photoinduced force, effects that are typically unaccounted for in simpler analytical models. Our findings show that the presence of the planar substrate and anisotropy of the tip have a substantial effect on the magnitude and the spectral response of the photoinduced force exerted on the tip. Unlike previous models, our calculations predict photoinduced forces that are within range of experimentally measured values in photoinduced force microscopy (PiFM) experiments.

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  • Received 11 January 2017
  • Revised 31 March 2017

DOI:https://doi.org/10.1103/PhysRevB.95.205440

©2017 American Physical Society

Physics Subject Headings (PhySH)

Atomic, Molecular & Optical

Authors & Affiliations

Faezeh Tork Ladani1 and Eric Olaf Potma2,1,*

  • 1Department of Electrical Engineering and Computer Science, University of California, Irvine, California 92697, USA
  • 2Department of Chemistry, University of California, Irvine, California 92697, USA

  • *epotma@uci.edu

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Vol. 95, Iss. 20 — 15 May 2017

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