Abstract
Neutron diffraction measurements were carried out on single crystals and powders of , where Yb moments form two interpenetrating planar sublattices of orthogonal dimers, a geometry known as Shastry-Sutherland lattice, and are stacked along the axis in a ladder geometry. orders antiferromagnetically at , and the magnetic structure determined from these measurements features the interleaving of two orthogonal sublattices into a magnetic supercell that is based on stripes with moments perpendicular to the dimer bonds, which are along and . Magnetic fields applied along or suppress the antiferromagnetic peaks from an individual sublattice, but leave the orthogonal sublattice unaffected, evidence for the Ising character of the Yb moments in that is supported by point charge calculations. Specific heat, magnetic susceptibility, and electrical resistivity measurements concur with neutron elastic scattering results that the longitudinal critical fluctuations are gapped with .
- Received 8 July 2014
- Revised 12 December 2015
DOI:https://doi.org/10.1103/PhysRevB.93.104419
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