High-field response of gated graphene at terahertz frequencies

Hadi Razavipour, Wayne Yang, Abdeladim Guermoune, Michael Hilke, David G. Cooke, Ibraheem Al-Naib, Marc M. Dignam, François Blanchard, Hassan A. Hafez, Xin Chai, Denis Ferachou, Tsuneyuki Ozaki, Pierre L. Lévesque, and Richard Martel

Phys. Rev. B 92, 245421 – Published 15 December 2015

Abstract

We study the Fermi energy level dependence of the nonlinear terahertz (THz) transmission of gated multilayer and single-layer graphene transferred onto sapphire and quartz substrates. The two samples represent two limits of low-field impurity scattering: short-range neutral and long-range charged impurity scattering, respectively. We observe an increase in the transmission as the field amplitude is increased due to intraband absorption bleaching starting at THz fields above 8 kV/cm. This effect arises from a field-induced reduction in THz conductivity that depends strongly on the Fermi energy. We account for intraband absorption using a free carrier Drude model that includes neutral and charged impurity scattering as well as optical phonon scattering. We find that although the Fermi-level dependence in the monolayer and five-layer samples is quite different due to the dominance of long- and short-range momentum scattering, respectively, both exhibit a strong dependence on the field amplitude that cannot be explained on the basis of an increase in the lattice temperature alone. Our results provide a deeper understanding of transport in graphene devices operating at THz frequencies and in modest kV/cm field strengths where nonlinearities exist.