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Short-range magnetic correlations in the highly correlated electron compound CeCu4Ga

B. G. Ueland, C. F. Miclea, K. Gofryk, Y. Qiu, F. Ronning, R. Movshovich, E. D. Bauer, J. S. Gardner, and J. D. Thompson
Phys. Rev. B 90, 121109(R) – Published 25 September 2014

Abstract

We present experimental results for the heavy-electron compound CeCu4Ga which show that it possesses short-range magnetic correlations down to a temperature of T=0.1 K. Our neutron scattering data show no evidence of long-range magnetic order occurring despite a peak in the specific heat at T*=1.2 K. Rather, magnetic diffuse scattering occurs which corresponds to short-range magnetic correlations occurring across two unit cells. The specific heat remains large as T0 K, resulting in a Sommerfeld coefficient of γ0=1.44(2) J/mol K2, and, below T*, the resistivity follows T2 behavior and the ac magnetic susceptibility becomes temperature independent. A magnetic peak centered at an energy transfer of Ec=0.24(1) meV is seen in inelastic neutron scattering data which shifts to higher energies and broadens under a magnetic field. We discuss the coexistence of large specific heat, magnetic fluctuations, and short-range magnetic correlations at low temperatures and compare our results to those for materials possessing spin-liquid behavior.

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  • Received 16 June 2014
  • Revised 27 August 2014

DOI:https://doi.org/10.1103/PhysRevB.90.121109

©2014 American Physical Society

Authors & Affiliations

B. G. Ueland1,2,3,*, C. F. Miclea1,4, K. Gofryk1,5, Y. Qiu6,7, F. Ronning1, R. Movshovich1, E. D. Bauer1, J. S. Gardner8, and J. D. Thompson1

  • 1Los Alamos National Laboratory, Los Alamos, New Mexico 87544, USA
  • 2Ames Laboratory, U.S. DOE, Iowa State University, Ames, Iowa 50011, USA
  • 3Department of Physics and Astronomy, Iowa State University, Ames, Iowa 50011, USA
  • 4National Institute of Materials Physics, 077125 Bucharest-Magurele, Romania
  • 5Idaho National Laboratory, Idaho Falls, Idaho 83415, USA
  • 6NIST Center for Neutron Research, National Institute of Standards and Technology, Gaithersburg, Maryland 20899, USA
  • 7Department of Materials Science and Engineering, University of Maryland, College Park, Maryland 20742, USA
  • 8National Synchrotron Radiation Research Center, Neutron Group, Hsinchu 30077, Taiwan

  • *bgueland@ameslab.gov; bgueland@gmail.com

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Issue

Vol. 90, Iss. 12 — 15 September 2014

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