Abstract
We present experimental results for the heavy-electron compound which show that it possesses short-range magnetic correlations down to a temperature of K. Our neutron scattering data show no evidence of long-range magnetic order occurring despite a peak in the specific heat at K. Rather, magnetic diffuse scattering occurs which corresponds to short-range magnetic correlations occurring across two unit cells. The specific heat remains large as K, resulting in a Sommerfeld coefficient of J/mol , and, below , the resistivity follows behavior and the ac magnetic susceptibility becomes temperature independent. A magnetic peak centered at an energy transfer of meV is seen in inelastic neutron scattering data which shifts to higher energies and broadens under a magnetic field. We discuss the coexistence of large specific heat, magnetic fluctuations, and short-range magnetic correlations at low temperatures and compare our results to those for materials possessing spin-liquid behavior.
- Received 16 June 2014
- Revised 27 August 2014
DOI:https://doi.org/10.1103/PhysRevB.90.121109
©2014 American Physical Society