Decoherence and lead-induced interdot coupling in nonequilibrium electron transport through interacting quantum dots: A hierarchical quantum master equation approach

R. Härtle, G. Cohen, D. R. Reichman, and A. J. Millis
Phys. Rev. B 88, 235426 – Published 20 December 2013

Abstract

The interplay between interference effects and electron-electron interactions in electron transport through an interacting double quantum dot system is investigated using a hierarchical quantum master equation approach which becomes exact if carried to infinite order and converges well if the temperature is not too low. Decoherence due to electron-electron interactions is found to give rise to pronounced negative differential resistance, enhanced broadening of structures in current-voltage characteristics, and an inversion of the electronic population. Dependence on gate voltage is shown to be a useful method of distinguishing decoherence-induced phenomena from effects induced by other mechanisms such as the presence of a blocking state. Comparison of results obtained by the hierarchical quantum master equation approach to those obtained from the Born-Markov approximation to the Nakajima-Zwanzig equation and from the noncrossing approximation to the nonequilibrium Green's function reveals the importance of an interdot coupling that originates from the energy dependence of the conduction bands in the leads and the need for a systematic perturbative expansion.

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  • Received 3 September 2013
  • Revised 6 November 2013

DOI:https://doi.org/10.1103/PhysRevB.88.235426

©2013 American Physical Society

Authors & Affiliations

R. Härtle1,*, G. Cohen2, D. R. Reichman2, and A. J. Millis1

  • 1Department of Physics, Columbia University, New York, New York 10027, USA
  • 2Department of Chemistry, Columbia University, New York, New York 10027, USA

  • *Institut für theoretische Physik, Georg-August-Universität Göttingen, Friedrich-Hund-Platz 1, D-37077 Göttingen, Germany.

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Issue

Vol. 88, Iss. 23 — 15 December 2013

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