Neutron scattering study of underdoped Ba1xKxFe2As2 (x=0.09 and 0.17) self-flux-grown single crystals and the universality of the tricritical point

C. R. Rotundu, W. Tian, K. C. Rule, T. R. Forrest, J. Zhao, J. L. Zarestky, and R. J. Birgeneau
Phys. Rev. B 85, 144506 – Published 4 April 2012

Abstract

We present a combination of elastic neutron scattering measurements in zero and 14.5 T and magnetization measurements in zero and 14 T on underdoped superconducting Ba1xKxFe2As2 (x=0.17), and the same measurements in zero field on a nonsuperconducting crystal with x=0.09. The data suggest that the underdoped materials may not be electronic phase separated but rather have slightly inhomogeneous potassium doping. The temperature dependence of the magnetic order parameter below the transition of the sample with x=0.09 is more gradual than that for the case of the undoped BaFe2As2, suggesting that this doping may be in the vicinity of a tricritical point. We advance therefore the hypothesis that the tricritical point is a common feature of all superconducting 122s. For the x=0.17 sample, while Tc is suppressed from 17 to 8 K by a magnetic field of 14 T, the intensity of the magnetic Bragg peaks (1 0 3) at 1.2 K is enhanced by 10%, showing competition of superconductivity and antiferromagnetism. The intensity of the magnetic Bragg peaks (1 0 3) in the (Tc, TN) temperature interval remain practically unchanged in 14.5 T within a 10% statistical error. The present results are discussed in the context of the existing literature.

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  • Received 14 November 2011

DOI:https://doi.org/10.1103/PhysRevB.85.144506

©2012 American Physical Society

Authors & Affiliations

C. R. Rotundu1,*, W. Tian2, K. C. Rule3, T. R. Forrest4, J. Zhao4, J. L. Zarestky2, and R. J. Birgeneau4,5

  • 1Materials Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, California 94720, USA
  • 2Ames Laboratory and Department of Physics and Astronomy, Iowa State University, Ames, Iowa 50011, USA
  • 3Helmholtz-Zentrum Berlin, Berlin, Germany
  • 4Department of Physics, University of California, Berkeley, California 94720, USA
  • 5Department of Materials Science and Engineering, University of California, Berkeley, California 94720, USA

  • *Author to whom correspondence should be addressed: CRRotundu@lbl.gov

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Vol. 85, Iss. 14 — 1 April 2012

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