Near-field optical studies of semicontinuous metal films

S. Ducourtieux, V. A. Podolskiy, S. Grésillon, S. Buil, B. Berini, P. Gadenne, A. C. Boccara, J. C. Rivoal, W. D. Bragg, K. Banerjee, V. P. Safonov, V. P. Drachev, Z. C. Ying, A. K. Sarychev, and Vladimir M. Shalaev
Phys. Rev. B 64, 165403 – Published 28 September 2001
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Abstract

Local field distributions in random metal-dielectric films near a percolation threshold are experimentally studied using scanning near-field optical microscopy (SNOM). The surface-plasmon oscillations in such percolation films are localized in small nanometer-scale areas, “hot spots,” where the local fields are much larger than the field of an incident electromagnetic wave. The spatial positions of the hot spots vary with the wavelength and polarization of the incident beam. Local near-field spectroscopy of the hot spots is performed using our SNOM. It is shown that the resonance quality-factor of hot spots increases from the visible to the infrared. Giant local optical activity associated with chiral plasmon modes has been obtained. The hot spot’s large local fields may result in local, frequency and spatially selective photomodification of percolation films.

  • Received 13 April 2001

DOI:https://doi.org/10.1103/PhysRevB.64.165403

©2001 American Physical Society

Authors & Affiliations

S. Ducourtieux1, V. A. Podolskiy2, S. Grésillon1, S. Buil3, B. Berini3, P. Gadenne3, A. C. Boccara1, J. C. Rivoal1, W. D. Bragg2, K. Banerjee2, V. P. Safonov4, V. P. Drachev5, Z. C. Ying2, A. K. Sarychev2, and Vladimir M. Shalaev6

  • 1CNRS UPR A0005 et Université P. et M. Curie, Laboratoire d’Optique Physique, ESPCI, 75231 Paris Cedex 05, France
  • 2Department of Physics, New Mexico State University, Las Cruces, New Mexico 88003
  • 3LMOV, Université de Versailles Saint-Quentin, 78035 Versailles, France
  • 4Institute of Automation and Electrometry, Novosibirsk 630090, Russia
  • 5Institute of Semiconductor Physics, Novosibirsk 630090, Russia
  • 6School of Electrical and Computer Engineering, Purdue University, West Lafayette, Indiana 47907-1285

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Issue

Vol. 64, Iss. 16 — 15 October 2001

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