Abstract
Using large single crystals (∼2 ), we have extended previous elastic and inelastic neutron scattering studies of the spin dynamics in the two-dimensional (2D) quantum antiferromagnet . We observe well-defined magnetic peaks for constant energy scans across the 2D magnetic rod for a wide range of temperatures and energies. The spectra are compared quantitatively with theoretical models. Simple spin-wave theory satisfactorily describes the experimental results well below . The thermal excitations of the low-energy (ħω≤3 meV) spectra, however, appear to deviate from the theory as is approached. The overall temperature and energy dependence of the spectra above (245–520 K) can be explained by the formula of Chakravarty, Halperin, Nelson, and Tyc for the dynamical structure factor S(q,ω) with no adjustable parameters. We do, however, observe a 2D elastic component which grows rapidly as is approached; it is hypothesized that this arises primarily from magnetic defects and is analogous to the ‘‘central peak’’ observed for many structural phase transitions.
- Received 10 May 1989
DOI:https://doi.org/10.1103/PhysRevB.40.4557
©1989 American Physical Society