Effect of pressure on impurity-impurity interactions in dilute Au:Mn, Cu:Mn, and Au:Fe spin-glass alloys

J. S. Schilling, P. J. Ford, U. Larsen, and J. A. Mydosh
Phys. Rev. B 14, 4368 – Published 15 November 1976
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Abstract

The electrical resistivity of the dilute spin-glass alloys Au-0.10-at.% Mn, 0.15-at.% Mn, 0.10-at.% Fe, 0.13-at.% Fe, and Cu-0.15-at.% Mn has been measured from 1.2 to 40 K at pressures to 100 kbar. In these alloys the cooperative "locking-in" of the impurity spins at a temperature T0 leads to a resistivity maximum at Tmax. Application of pressure is found to shift Tmax in a manner which is strongly system dependent: dTmaxdP>0 for Au:Mn, dTmaxdP0 for Cu:Mn, and dTmaxdP<0 for Au:Fe. These results are shown to be clearly incompatible with the widely held belief that kTmaxΔRKKY, where ΔRKKYcJ2S(S+1)EF is the average strength of the Ruderman-Kittel-Kasuya-Yosida interaction, and indicate that Tmax is a function of both ΔRKKY and TK, the Kondo temperature. This expectation is confirmed in a recent theory of Larsen who introduces an impurity-impurity interaction strength Δc into the parquet approximation of the Kondo resistivity and obtains an explicit expression for Tmax=Tmax(Δc,TK). It is shown that both the sign and the magnitude of dTmaxdP for the systems studied here are a natural consequence of both increasing TK and Δc in all systems and depend on the relative magnitudes of Δc and TK. In particular, one would expect to find dTmaxdP<0 in systems such as Au:Fe with relatively high Kondo temperatures. A further result of the analysis is that Δc(P)ΔRKKY(P), lending support to the view that in these systems the long-range RKKY oscillations represent the dominant impurity-impurity interaction mechanism.

  • Received 12 February 1976

DOI:https://doi.org/10.1103/PhysRevB.14.4368

©1976 American Physical Society

Authors & Affiliations

J. S. Schilling and P. J. Ford

  • Institut für Experimentalphysik IV, Universität Bochum, 463 Bochum, Germany

U. Larsen

  • Physics Laboratory I, H. C. Ørsted Institute, University of Copenhagen, DK-2100 Copenhagen, Denmark

J. A. Mydosh*

  • Institut für Festkörperforschung, Kernforschungsanlage Jülich, 517 Jülich, Germany

  • *Present address: Kamerlingh Onnes Laboratorium der Rijks-Universiteit, Leiden, The Netherlands.

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Vol. 14, Iss. 10 — 15 November 1976

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