Crossover from weakly indirect to direct excitons in atomically thin films of InSe

Adrián Ceferino, Kok Wee Song, Samuel J. Magorrian, Viktor Zólyomi, and Vladimir I. Fal'ko
Phys. Rev. B 101, 245432 – Published 22 June 2020
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Abstract

We perform a k·p theory analysis of the spectra of the lowest energy and excited states of the excitons in few-layer atomically thin films of InSe taking into account in plane electric polarizability of the film and the influence of the encapsulation environment. For the thinner films, the lowest-energy state of the exciton is weakly indirect in momentum space, with its dispersion showing minima at a layer-number-dependent wave number, due to an inverted edge of a relatively flat topmost valence band branch of the InSe film spectrum, and we compute the activation energy from the momentum dark exciton ground state into the bright state. For the films with more than seven In2Se2 layers, the exciton dispersion minimum shifts to Γ point.

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  • Received 14 January 2020
  • Accepted 23 March 2020

DOI:https://doi.org/10.1103/PhysRevB.101.245432

©2020 American Physical Society

Physics Subject Headings (PhySH)

Condensed Matter, Materials & Applied Physics

Authors & Affiliations

Adrián Ceferino1,2,*, Kok Wee Song2,†, Samuel J. Magorrian2, Viktor Zólyomi3, and Vladimir I. Fal'ko1,2,4

  • 1Department of Physics and Astronomy, University of Manchester, Oxford Road, Manchester, M13 9PL, United Kingdom
  • 2National Graphene Institute, Booth Street East, Manchester, M13 9PL, United Kingdom
  • 3STFC Hartree Centre, Daresbury Laboratory, Daresbury, Warrington, WA4 4AD, United Kingdom
  • 4Henry Royce Institute for Advanced Materials, Manchester, M13 9PL, United Kingdom

  • *adrian.ceferino@postgrad.manchester.ac.uk
  • kokwee.song@manchester.ac.uk

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Issue

Vol. 101, Iss. 24 — 15 June 2020

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