Antiferromagnetic Order with Spatially Inhomogeneous Ordered Moment Size of Zn- and Si-Doped CuGeO3

K. M. Kojima, Y. Fudamoto, M. Larkin, G. M. Luke, J. Merrin, B. Nachumi, Y. J. Uemura, M. Hase, Y. Sasago, K. Uchinokura, Y. Ajiro, A. Revcolevschi, and J.-P. Renard
Phys. Rev. Lett. 79, 503 – Published 21 July 1997
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Abstract

We report muon spin relaxation measurements of the doped spin-Peierls system (Cu1xZnx)(Ge1ySiy)O3. Spontaneous muon spin precession in zero applied field was observed, confirming the presence of antiferromagnetic order in this series of compounds. In contrast to usual antiferromagnets, muon spin precession is accompanied by a relaxation signal indicating a large spatial inhomogeneity of the ordered moment size. Assuming an exponential decay of the moment size away from the doping centers, we estimated a decay length of ξ10 lattice units along the chain. We suggest that both Zn and Si doping induces the same maximum moment size around the doping center.

  • Received 10 January 1997

DOI:https://doi.org/10.1103/PhysRevLett.79.503

©1997 American Physical Society

Authors & Affiliations

K. M. Kojima1, Y. Fudamoto1, M. Larkin1, G. M. Luke1, J. Merrin1, B. Nachumi1, Y. J. Uemura1, M. Hase2, Y. Sasago2, K. Uchinokura2, Y. Ajiro3, A. Revcolevschi4, and J.-P. Renard5

  • 1Department of Physics, Columbia University, New York, New York 10027
  • 2Department of Applied Physics, University of Tokyo, Tokyo 113, Japan
  • 3Department of Applied Physics, Fukui University, Fukui 910, Japan
  • 4Laboratoire de Chimie des Solides, Université Paris-Sud, 91405 Orsay, Cédex, France
  • 5Institut d'Electronique Fondamentale, Université Paris-Sud, 91405 Orsay Cédex, France

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Vol. 79, Iss. 3 — 21 July 1997

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