Microscopic Origin of Internal Stresses in Jammed Soft Particle Suspensions

Lavanya Mohan, Roger T. Bonnecaze, and Michel Cloitre
Phys. Rev. Lett. 111, 268301 – Published 26 December 2013

Abstract

The long time persistence of mechanical stresses is a generic property of glassy materials. Here we identify the microscopic mechanisms that control internal stresses in highly concentrated suspensions of soft particles brought to rest from steady flow. The persistence of the asymmetric angular distortions which characterize the pair distribution function during flow is at the origin of the internal stresses. Their long time evolution is driven by in-cage rearrangements of the elastic contacts between particles. The trapped macroscopic stress is related to the solvent viscosity, particle elasticity and volume fraction through a universal scaling derived from simulations and experiments.

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  • Received 14 August 2013

DOI:https://doi.org/10.1103/PhysRevLett.111.268301

© 2013 American Physical Society

Authors & Affiliations

Lavanya Mohan*, Roger T. Bonnecaze*, and Michel Cloitre

  • *Department of Chemical Engineering and Texas Materials Institute, The University of Texas at Austin, Austin, Texas 78712, USA
  • Matière Molle et Chimie (UMR 7167, ESPCI-CNRS), ESPCI ParisTech 10 rue Vauquelin, 75005 Paris, France

  • *rtb@che.utexas.edu
  • *michel.cloitre@espci.fr

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Vol. 111, Iss. 26 — 27 December 2013

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