Elastic Signature of Flow Events in Supercooled Liquids Under Shear

Joyjit Chattoraj and Anaël Lemaître
Phys. Rev. Lett. 111, 066001 – Published 8 August 2013
PDFHTMLExport Citation

Abstract

Using numerical simulation of a 2D Lennard-Jones system, we study the crossover from shear thinning to Newtonian flow. We find that the short-time elastic response of our system essentially does not change through this crossover, and show that, in the Newtonian regime, thermal activation triggers shear transformations, i.e., local irreversible shear events that produce Eshelby (long-ranged, anisotropic) deformation fields as previously seen in low-T glasses. Quite surprisingly, these Eshelby fields are found to persist much beyond the α-relaxation time, and shear thinning to coincide with the emergence of correlations between shear relaxation centers.

  • Figure
  • Figure
  • Figure
  • Figure
  • Figure
  • Received 6 November 2012

DOI:https://doi.org/10.1103/PhysRevLett.111.066001

© 2013 American Physical Society

Authors & Affiliations

Joyjit Chattoraj1,2 and Anaël Lemaître1

  • 1Laboratoire Navier (UMR 8205), Université Paris-Est, CNRS, ENPC, IFSTTAR, F-77420 Marne-la-Valle, France
  • 2Institute of Physical Chemistry, University of Münster, Corrensstrasse 30, D-48149 Münster, Germany

Article Text (Subscription Required)

Click to Expand

Supplemental Material (Subscription Required)

Click to Expand

References (Subscription Required)

Click to Expand
Issue

Vol. 111, Iss. 6 — 9 August 2013

Reuse & Permissions
Access Options
Author publication services for translation and copyediting assistance advertisement

Authorization Required


×
×

Images

×

Sign up to receive regular email alerts from Physical Review Letters

Log In

Cancel
×

Search


Article Lookup

Paste a citation or DOI

Enter a citation
×