Tailoring Light-Matter Interaction with a Nanoscale Plasmon Resonator

Nathalie P. de Leon, Brendan J. Shields, Chun L. Yu, Dirk E. Englund, Alexey V. Akimov, Mikhail D. Lukin, and Hongkun Park
Phys. Rev. Lett. 108, 226803 – Published 31 May 2012
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Abstract

We propose and demonstrate a new approach for achieving enhanced light-matter interactions with quantum emitters. Our approach makes use of a plasmon resonator composed of defect-free, highly crystalline silver nanowires surrounded by patterned dielectric distributed Bragg reflectors. These resonators have an effective mode volume (Veff) 2 orders of magnitude below the diffraction limit and a quality factor (Q) approaching 100, enabling enhancement of spontaneous emission rates by a factor exceeding 75 at the cavity resonance. We also show that these resonators can be used to convert a broadband quantum emitter to a narrow-band single-photon source with color-selective emission enhancement.

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  • Received 3 February 2012

DOI:https://doi.org/10.1103/PhysRevLett.108.226803

© 2012 American Physical Society

Authors & Affiliations

Nathalie P. de Leon1,2, Brendan J. Shields2, Chun L. Yu1, Dirk E. Englund2,*, Alexey V. Akimov2,3,4, Mikhail D. Lukin2,†, and Hongkun Park1,2,‡

  • 1Department of Chemistry and Chemical Biology, Harvard University, Cambridge, Massachusetts 02138, USA
  • 2Department of Physics, Harvard University, Cambridge, Massachusetts 02138, USA
  • 3Lebedev Institute of Physics, Moscow, Russia
  • 4Russian Quantum Center, Moscow, Russia

  • *Present address: Department of Electrical Engineering, Columbia University, New York, NY 10027, USA.
  • To whom correspondence should be addressed. hongkun_park@harvard.edu
  • lukin@physics.harvard.edu

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Issue

Vol. 108, Iss. 22 — 1 June 2012

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