Direct and third-body mediated resonance energy transfer in dimensionally constrained nanostructures

Dilusha Weeraddana, Malin Premaratne, and David L. Andrews
Phys. Rev. B 92, 035128 – Published 14 July 2015

Abstract

The process of resonance energy transfer (RET) in a nanostructure influenced by a vicinal, nonabsorbing third body is studied within the framework of molecular quantum electrodynamics. Direct RET and the influence of neighboring matter have been studied previously, mainly for molecules. However, a complete study or unified understanding of direct and indirect RET in nanostructures with different dimensionalities is still lacking. Therefore, there is a strong need for a complete theory that models RET for the cases of quantum wells, nanowires, and quantum dots. We construct a detailed picture of excitation energy transfer in nanostructures and how it is affected by another quantum object, which includes the derivation of quantum amplitudes based on second- and fourth-order time-dependent perturbation theories, and the derivation of transfer rates and distance dependencies, providing a complete picture and understanding of RET in nanostructures. The results of the derivations indicate that the dimensionality of the nanostructure determines the controllability of the RET rate. Furthermore, third-body mediation leads to a nonvanishing RET in the coupling of nanowire to nanowire and quantum dot to quantum dot.

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  • Received 4 March 2015
  • Revised 13 May 2015

DOI:https://doi.org/10.1103/PhysRevB.92.035128

©2015 American Physical Society

Authors & Affiliations

Dilusha Weeraddana* and Malin Premaratne

  • Advanced Computing and Simulation Laboratory (AχL), Department of Electrical and Computer Systems Engineering, Monash University, Clayton, Victoria 3800, Australia

David L. Andrews

  • School of Chemistry, University of East Anglia, Norwich Research Park, Norwich NR4 7TJ, United Kingdom

  • *dilusha.weeraddana@monash.edu
  • malin.premaratne@monash.edu
  • d.l.andrews@uea.ac.uk

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Issue

Vol. 92, Iss. 3 — 15 July 2015

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