Symmetry and correlations underlying hidden order in URu2Si2

Nicholas P. Butch, Michael E. Manley, Jason R. Jeffries, Marc Janoschek, Kevin Huang, M. Brian Maple, Ayman H. Said, Bogdan M. Leu, and Jeffrey W. Lynn
Phys. Rev. B 91, 035128 – Published 26 January 2015
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Abstract

We experimentally investigate the symmetry in the hidden order (HO) phase of intermetallic URu2Si2 by mapping the lattice and magnetic excitations via inelastic neutron and x-ray scattering measurements in the HO and high-temperature paramagnetic phases. At all temperatures, the excitations respect the zone edges of the body-centered tetragonal paramagnetic phase, showing no signs of reduced spatial symmetry, even in the HO phase. The magnetic excitations originate from transitions between hybridized bands and track the Fermi surface, whose features are corroborated by the phonon measurements. Due to a large hybridization energy scale, a full uranium moment persists in the HO phase, consistent with a lack of observed crystal-field-split states. Our results are inconsistent with local order-parameter models and the behavior of typical density waves. We suggest that an order parameter that does not break spatial symmetry would naturally explain these characteristics.

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  • Received 6 June 2014
  • Revised 1 November 2014

DOI:https://doi.org/10.1103/PhysRevB.91.035128

©2015 American Physical Society

Authors & Affiliations

Nicholas P. Butch1,2,3,*, Michael E. Manley4, Jason R. Jeffries3, Marc Janoschek5,6, Kevin Huang6, M. Brian Maple6, Ayman H. Said7, Bogdan M. Leu7, and Jeffrey W. Lynn2

  • 1Center for Nanophysics and Advanced Materials, Department of Physics, University of Maryland, College Park, Maryland 20742, USA
  • 2NIST Center for Neutron Research, National Institute of Standards and Technology, 100 Bureau Drive, Gaithersburg, Maryland 20899, USA
  • 3Lawrence Livermore National Laboratory, 7000 East Ave., Livermore, California 94550, USA
  • 4Oak Ridge National Laboratory, Oak Ridge, Tennessee 37831, USA
  • 5Los Alamos National Laboratory, Los Alamos, New Mexico 87545, USA
  • 6Department of Physics, University of California-San Diego, 9500 Gilman Drive, La Jolla, California 92093, USA
  • 7Advanced Photon Source, Argonne National Laboratory, 9700 S. Cass Ave., Argonne, Illinois 60439, USA

  • *nicholas.butch@nist.gov

See Also

Lattice dynamics of the heavy-fermion compound URu2Si2

J. Buhot, M. A. Méasson, Y. Gallais, M. Cazayous, A. Sacuto, F. Bourdarot, S. Raymond, G. Lapertot, D. Aoki, L. P. Regnault, A. Ivanov, P. Piekarz, K. Parlinski, D. Legut, C. C. Homes, P. Lejay, and R. P. S. M. Lobo
Phys. Rev. B 91, 035129 (2015)

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Vol. 91, Iss. 3 — 15 January 2015

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