Local-field effect on the spontaneous radiative emission rate

Chang-Kui Duan, Hongli Wen, and Peter A. Tanner
Phys. Rev. B 83, 245123 – Published 24 June 2011

Abstract

The effect of the dielectric medium upon the spontaneous emission rate was investigated using lead borate glass of various compositions lightly doped with the Eu3+ lanthanide ion. A dual approach used the variation of (i) electric dipole/magnetic dipole (ED/MD) emission rates from spectral integrations and (ii) absolute ED emission rates from lifetime measurements for comparison with the variation of the refractive index of the glass medium. Contrary to a previous study [Phys. Rev. Lett. 91, 203903 (2003)], the results show the relevance of the virtual-cavity model in this case. The MD emission rates were taken to follow the n3 increase in density of photon states in the medium. The justifications for employing Eu3+ for identifying the appropriate model are given.

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  • Received 21 April 2011

DOI:https://doi.org/10.1103/PhysRevB.83.245123

©2011 American Physical Society

Authors & Affiliations

Chang-Kui Duan*, Hongli Wen, and Peter A. Tanner

  • Department of Biology and Chemistry, City University of Hong Kong, Tat Chee Avenue, Kowloon, Hong Kong S.A.R., People's Republic of China

  • *Present address: Department of Physics, University of Science and Technology of China, Hefei, Anhui 230026, People's Republic of China.
  • bhtan@cityu.edu.hk

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Vol. 83, Iss. 24 — 15 June 2011

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