Tunable Bose-Einstein condensation and rotonlike excitation spectra with dipolar exciton-polaritons in crossed fields

Timofey V. Maximov, I. L. Kurbakov, Nina S. Voronova, and Yurii E. Lozovik
Phys. Rev. B 108, 195304 – Published 13 November 2023

Abstract

We develop the many-body theory of dipolar exciton-polaritons in an optical microcavity in crossed out-of-plane electric and in-plane magnetic fields. Even for relatively weak fields, we reveal the existence of two minima in the bare lower-polariton dispersion, which give rise to the tunable transition between the polariton Bose-Einstein condensate and that of excitons, produced by the competition between these minima. We predict that such dipolar condensate exhibits a roton-maxon character of the excitation spectrum, never before observed for polaritons. We show that upon the transition between the two condensation regimes, the weak correlations in the polariton gas give way to the intermediate interparticle correlations characteristic for excitons, and that the transition is accompanied by a sharp quenching of photoluminescence as the lifetime is increased by several orders of magnitude. While in the polariton regime, the luminescence peak corresponding to the condensate is shifted to a nonzero angle. The angular dependence of the two-photon decay time in the Hanbury Brown and Twiss experiment is calculated and used as a tool to evidence the formation of the macroscopically coherent state. Our proposal opens opportunities towards manipulating the superfluid properties and extended-range dipole-dipole correlations of exciton-polariton condensates.

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  • Received 6 June 2023
  • Revised 17 October 2023
  • Accepted 18 October 2023

DOI:https://doi.org/10.1103/PhysRevB.108.195304

©2023 American Physical Society

Physics Subject Headings (PhySH)

Condensed Matter, Materials & Applied Physics

Authors & Affiliations

Timofey V. Maximov1,2, I. L. Kurbakov3, Nina S. Voronova4,5,*, and Yurii E. Lozovik3,6,†

  • 1National Research University “Moscow Institute of Physics and Technology”, Phystech School of Fundamental and Applied Physics, 141700 Dolgoprudny, Moscow Region, Russia
  • 2N. L. Dukhov Research Institute of Automatics (VNIIA), 127055 Moscow, Russia
  • 3Institute for Spectroscopy RAS, 142190 Troitsk, Moscow, Russia
  • 4National Research Nuclear University MEPhI (Moscow Engineering Physics Institute), 115409 Moscow, Russia
  • 5Russian Quantum Center, Skolkovo IC, Bolshoy boulevard 30 bld. 1, 121205 Moscow, Russia
  • 6National Research University Higher School of Economics, 109028 Moscow, Russia

  • *nsvoronova@mephi.ru
  • lozovik@isan.troitsk.ru

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Issue

Vol. 108, Iss. 19 — 15 November 2023

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