Incommensurate magnetic order in the Z2 kagome metal GdV6Sn6

Zach Porter, Ganesh Pokharel, Jong-Woo Kim, Phillip J. Ryan, and Stephen D. Wilson
Phys. Rev. B 108, 035134 – Published 18 July 2023
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Abstract

We characterize the magnetic ground state of the topological kagome metal GdV6Sn6 via resonant x-ray diffraction. Previous magnetoentropic studies of GdV6Sn6 suggested the presence of a modulated magnetic order distinct from the ferromagnetism that is easily polarized by the application of a magnetic field. Diffraction data near the Gd-L2 edge directly resolve a c-axis modulated spin structure order on the Gd sublattice with an incommensurate wave vector that evolves upon cooling toward a partial lock-in transition. While equal moment (spiral) and amplitude (sine) modulated spin states cannot be unambiguously discerned from the scattering data, the overall phenomenology suggests an amplitude modulated state with moments predominantly oriented in the ab plane. Comparisons to the “double-flat” spiral state observed in Mn-based RMn6Sn6 kagome compounds of the same structure type are discussed.

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  • Received 21 April 2023
  • Accepted 26 June 2023

DOI:https://doi.org/10.1103/PhysRevB.108.035134

©2023 American Physical Society

Physics Subject Headings (PhySH)

Condensed Matter, Materials & Applied Physics

Authors & Affiliations

Zach Porter1,2, Ganesh Pokharel1, Jong-Woo Kim3, Phillip J. Ryan3, and Stephen D. Wilson1,4,*

  • 1Materials Department, University of California, Santa Barbara, California 93106, USA
  • 2Linac Coherent Light Source and Stanford Institute for Materials and Energy Sciences, SLAC National Accelerator Laboratory, Menlo Park, California 94025, USA
  • 3X-ray Science Division, Argonne National Laboratory, Argonne, Illinois 60439, USA
  • 4California Nanosystems Institute, University of California, Santa Barbara, California 93106, USA

  • *stephendwilson@ucsb.edu

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Issue

Vol. 108, Iss. 3 — 15 July 2023

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