• Rapid Communication

Magnetic-field-induced splitting and polarization of monolayer-based valley exciton polaritons

N. Lundt, M. Klaas, E. Sedov, M. Waldherr, H. Knopf, M. Blei, S. Tongay, S. Klembt, T. Taniguchi, K. Watanabe, U. Schulz, A. Kavokin, S. Höfling, F. Eilenberger, and C. Schneider
Phys. Rev. B 100, 121303(R) – Published 27 September 2019

Abstract

Atomically thin crystals of transition-metal dichalcogenides are ideally suited to study the interplay of light-matter coupling, polarization, and magnetic field effects. In this Rapid Communication, we investigate the formation of exciton polaritons in a MoSe2 monolayer, which is integrated in a fully grown, monolithic microcavity. Due to the narrow linewidth of the polaritonic resonances, we are able to directly investigate the emerging valley Zeeman splitting of the hybrid light-matter resonances in the presence of a magnetic field. At a detuning of 54.5 meV (13.5% matter constituent of the lower polariton branch), we find a Zeeman splitting of the lower polariton branch of 0.36 meV, which can be directly associated with an excitonic g-factor of 3.94±0.13. Remarkably, we find that a magnetic field of 6 T is sufficient to induce a notable valley polarization of 15% in our polariton system, which approaches 30% at 9 T. This circular polarization degree of the polariton (ground) state exceeds the polarization of the exciton reservoir for equal magnetic field magnitudes by approximately 50%, which is a clear hint of valley-dependent bosonic stimulation in our strongly coupled system in the subthreshold, fluctuation-dominated regime.

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  • Received 13 December 2018
  • Revised 7 August 2019

DOI:https://doi.org/10.1103/PhysRevB.100.121303

©2019 American Physical Society

Physics Subject Headings (PhySH)

Condensed Matter, Materials & Applied Physics

Authors & Affiliations

N. Lundt1, M. Klaas1, E. Sedov2,3, M. Waldherr1, H. Knopf4,5,6, M. Blei7, S. Tongay7, S. Klembt1, T. Taniguchi8, K. Watanabe8, U. Schulz4, A. Kavokin9,10,2, S. Höfling1,11, F. Eilenberger4,5,6, and C. Schneider1

  • 1Technische Physik, Wilhelm-Conrad-Röntgen-Research Center for Complex Material Systems, Universität Würzburg, Am Hubland, D-97074 Würzburg, Germany
  • 2School of Physics and Astronomy, University of Southampton, Highfield, Southampton SO17 1BJ, United Kingdom
  • 3Vladimir State University named after A. G. and N. G. Stoletovs, Gorky Street 87, 600000 Vladimir, Russia
  • 4Fraunhofer-Institute for Applied Optics and Precision Engineering IOF, Center of Excellence in Photonics, Albert-Einstein-Straße 7, D-07745 Jena, Germany
  • 5Institute of Applied Physics, Abbe Center of Photonics, Friedrich Schiller University, Albert-Einstein-Straße 15, D-07745 Jena, Germany
  • 6Fraunhofer-Institute for Applied Optics and Precision Engineering IOF, Max Planck School of Photonics, Albert-Einstein-Straße 7, D-07745 Jena, Germany
  • 7School for Engineering of Matter, Transport, and Energy, Arizona State University, Tempe, Arizona 85287, USA
  • 8National Institute for Materials Science, Tsukuba, Ibaraki 305-0044, Japan
  • 9Westlake University, 18 Shilongshan Road, Hangzhou 310024, Zhejiang Province, China
  • 10Institute of Natural Sciences, Westlake Institute for Advanced Study, 18 Shilongshan Road, Hangzhou 310024, Zhejiang Province, China
  • 11SUPA, School of Physics and Astronomy, University of St. Andrews, St. Andrews KY16 9SS, United Kingdom

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Issue

Vol. 100, Iss. 12 — 15 September 2019

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