Tunneling current induced squeezing of the single-molecule vibrational mode

N. S. Maslova, V. N. Mantsevich, P. I. Arseyev, and I. M. Sokolov
Phys. Rev. B 100, 035307 – Published 16 July 2019

Abstract

A tunneling system with a molecule between the leads was analyzed in the framework of the adiabatic approach. The adiabatic approach allowed us to consider effects of equilibrium ion positions changing and vibrational mode frequency modification due to the electrons tunneling through the molecule localized states. It was demonstrated that vibrational states become squeezed if the tunneling current flows through the molecule. The mean-square displacement of the molecule and the degree of squeezing depend on the system parameters and could be tuned by applied bias voltage. Obtained results demonstrate the possibility of molecule ions' effective “freezing” by the tunneling current.

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  • Received 20 March 2019
  • Revised 2 June 2019

DOI:https://doi.org/10.1103/PhysRevB.100.035307

©2019 American Physical Society

Physics Subject Headings (PhySH)

Condensed Matter, Materials & Applied PhysicsAtomic, Molecular & Optical

Authors & Affiliations

N. S. Maslova1, V. N. Mantsevich2, P. I. Arseyev3, and I. M. Sokolov4

  • 1Chair of Quantum Electronics and Quantum Technology Center, Physics Department, Lomonosov Moscow State University, 119991 Moscow, Russia
  • 2Chair of Semiconductors and Cryoelectronics and Quantum Technology Center, Physics Department, Lomonosov Moscow State University, 119991 Moscow, Russia
  • 3P. N. Lebedev Physical Institute RAS, 119991 Moscow, Russia
  • 4Institut fur Physik and IRIS Adlesdorf, Humboldt Universitat zu Berlin, Newtonstrasse 15, 12489 Berlin, Germany

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Issue

Vol. 100, Iss. 3 — 15 July 2019

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