Coherent control of two-state systems is traditionally achieved by resonant pulses of specific Rabi frequency and duration, by adiabatic techniques using level crossings or delayed pulses, or by sequences of pulses with precise relative phases (composite pulses). Here we develop a method for high-fidelity coherent control which uses a sequence of detuning pulses. By using the detuning pulse areas as control parameters, and driving on an analogy with composite pulses, we report a great variety of detuning pulse sequences for broadband and narrow-band transition probability profiles.

• Received 19 June 2018
• Revised 25 September 2018

DOI:https://doi.org/10.1103/PhysRevA.99.013424