Issue 46, 2022

3D-structured mesoporous silica memristors for neuromorphic switching and reservoir computing

Abstract

Memristors are emerging as promising candidates for practical application in reservoir computing systems that are capable of temporal information processing. Here, we experimentally implement a physical reservoir computing system using resistive memristors based on three-dimensional (3D)-structured mesoporous silica (mSiO2) thin films fabricated by a low cost, fast and vacuum-free sol–gel technique. The in situ learning capability and a classification accuracy of 100% on a standard machine learning dataset are experimentally demonstrated. The volatile (temporal) resistive switching in diffusive memristors arises from the formation and subsequent spontaneous rupture of conductive filaments via diffusion of Ag species within the 3D-structured nanopores of the mSiO2 thin film. Besides volatile switching, the devices also exhibit a bipolar non-volatile resistive switching behavior when the devices are operated at a higher compliance current level. The implementation of mSiO2 thin films opens the route to fabricate a simple and low cost dynamic memristor with a temporal information process functionality, which is essential for neuromorphic computing applications.

Graphical abstract: 3D-structured mesoporous silica memristors for neuromorphic switching and reservoir computing

Supplementary files

Article information

Article type
Communication
Submitted
12 Sep 2022
Accepted
10 Nov 2022
First published
10 Nov 2022
This article is Open Access
Creative Commons BY license

Nanoscale, 2022,14, 17170-17181

3D-structured mesoporous silica memristors for neuromorphic switching and reservoir computing

A. H. Jaafar, L. Shao, P. Dai, T. Zhang, Y. Han, R. Beanland, N. T. Kemp, P. N. Bartlett, A. L. Hector and R. Huang, Nanoscale, 2022, 14, 17170 DOI: 10.1039/D2NR05012A

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