PbSrSiO4: a new ultraviolet nonlinear optical material with a strong second harmonic generation response and moderate birefringence

Shutong Jiang; Jinjie Zhou; Hongping Wu; Hongwei Yu; Zhanggui Hu; Jiyang Wang; Yicheng Wu

doi:10.1039/D0CC02123G

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PbSrSiO₄: a new ultraviolet nonlinear optical material with a strong second harmonic generation response and moderate birefringence†

Shutong Jiang,^a Jinjie Zhou,^a Hongping Wu,

*^a Hongwei Yu,

*^a Zhanggui Hu,^a Jiyang Wang^a and Yicheng Wu^a

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* Corresponding authors

^a Tianjin Key Laboratory of Functional Crystal Materials, Institute of Functional Crystal, Tianjin University of Technology, Tianjin 300384, China
E-mail: wuhp@ms.xjb.ac.cn

Abstract

Introduction of Pb²⁺ cations in silicate systems generates a new compound, PbSrSiO₄, which exhibits excellent properties, including a strong second harmonic generation response (∼5.8 × KDP), a short UV cut-off edge (240 nm) and moderate birefringence (0.053@1064 nm). These results suggest that PbSrSiO₄ is a promising UV NLO material.

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Article information

DOI: https://doi.org/10.1039/D0CC02123G
Article type: Communication
Submitted: 23 Mar 2020
Accepted: 15 May 2020
First published: 18 May 2020

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Chem. Commun., 2020,56, 7104-7107

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PbSrSiO₄: a new ultraviolet nonlinear optical material with a strong second harmonic generation response and moderate birefringence

S. Jiang, J. Zhou, H. Wu, H. Yu, Z. Hu, J. Wang and Y. Wu, Chem. Commun., 2020, 56, 7104 DOI: 10.1039/D0CC02123G

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Chemical Communications